典型文献
Facile Synthesis and High-Value Utilization of Ammonia
文献摘要:
Ammonia is a key component in fertilizer and the carbon-free hydrogen carrier.Catalytic ammonia synthesis and utilization have played a central role in the development of chemical engineering.The industrial production of ammonia remains dependent on the energy-and carbon-intensive Haber-Bosch process.A major effort has been devoted to developing robust and efficient catalysts,as well as alternative benign processes.Herein,we detail our endeavors that develop the ammonia synthesis and decomposition catalysts,and utilize the ammonia energy.We firstly discuss the catalysts for ammonia synthesis via dissociative and associative process,and the regulation of catalysts'properties.Then,we review the burgeoning electrocata-lytic nitrogen reduction process,focusing on the enhanced catalytic performances by the regulation of the catalysts and the electrode.Additionally,we provide a novel high-value utilization of ammonia to achieve the"zero-carbon"circular economy.The promising catalysts,reactors,and ammonia energy systems have been discussed in detail.We end this Account that offers future research directions and prospects of ammonia.
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作者姓名:
Yu Luo;Shijing Liang;Xiuyun Wang;Bingyu Lin;Chongqi Chen;Lilong Jiang
作者机构:
National Engineering Research Center of Chemical Fertilizer Catalyst,Fuzhou University,Fuzhou,Fujian 350002,China;Qingyuan Innovation Laboratory,Quanzhou,Fujian 362801,China
文献出处:
引用格式:
[1]Yu Luo;Shijing Liang;Xiuyun Wang;Bingyu Lin;Chongqi Chen;Lilong Jiang-.Facile Synthesis and High-Value Utilization of Ammonia)[J].中国化学(英文版),2022(08):953-964
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0.621497
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