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Green Synthesis of Nitrogen-to-Ammonia Fixation:Past,Present,and Future
文献摘要:
The nitrogen(N2)-to-ammonia(NH3)fixation driven by renewable energy has an attractive prospect to relieve the global warming and reduce the consumption of fossil fuels.Ideally,photocatalytic,electrochemical,and photoelectrochemical approaches are developed as the next-generation NH3 synthesis technologies to substitute the Haber-Bosch method.However,the NH3 yield rate of nitrogen reduction reaction(NRR)by green approaches is extremely low,resulting in the current dilemma of NRR and contamination issues.Thus,in this mini review,the past advances on the sustainable NRR are briefly summarized in the three aspects as follows:the selectivity and adjustment of various catalysts,the type of electrolyte/solvent system,and the investigation of reaction conditions.Subsequently,the recent critical activities in the area of sustainable NH3 synthesis are analyzed and discussed deeply,and a perspective for rational and healthy development of this area is provided positively.
文献关键词:
作者姓名:
Jianyun Zheng;Li Jiang;Yanhong Lyu;San Ping Jiang;Shuangyin Wang
作者机构:
State Key Laboratory of Chem/Bio-Sensing and Chemometrics,College of Chemistry and Chemical Engineering,Hunan University,Changsha 410082,China;Department of Educational Science,Hunan First Normal University,Changsha 410205,China;Curtin University,Perth WA,Australia
引用格式:
[1]Jianyun Zheng;Li Jiang;Yanhong Lyu;San Ping Jiang;Shuangyin Wang-.Green Synthesis of Nitrogen-to-Ammonia Fixation:Past,Present,and Future)[J].能源与环境材料(英文),2022(02):452-457
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AB值:
0.706255
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