典型文献
Rational Manipulation of Intermediates on Copper for CO2 Electroreduction Toward Multicarbon Products
文献摘要：
Excess greenhouse gas emissions, primarily carbon dioxide (CO2 ), have caused major environmental concerns worldwide. The electroreduction of CO2 into valuable chemicals using renewable energy is an ecofriendly approach to achieve carbon neutrality. In this regard, copper (Cu) has attracted considerable attention as the only known metallic catalyst available for converting CO2 to high-value multicarbon (C 2+ ) products. The production of C 2+ involves complicated C–C coupling steps and thus imposes high demands on intermediate regulation. In this review, we discuss multiple strategies for modulating intermediates to facilitate C 2+ formation on Cu-based catalysts. Furthermore, several sophisticated insitu characterization techniques are outlined for elucidating the mechanism of C–C coupling. Lastly, the challenges and future directions of CO2 electroreduction to C 2+ are envisioned.
文献关键词：
中图分类号：
作者姓名：
Guangyi Jiang;Daliang Han;Zishan Han;Jiachen Gao;Xinyu Wang;Zhe Weng;Quan-Hong Yang
作者机构：
Nanoyang Group,State Key Laboratory of Chemical Engineering,School of Chemical Engineering and Technology,Tianjin University,Tianjin 300072,China;Haihe Laboratory of Sustainable Chemical Transformations, Tianjin 300192,China;Collaborative Innovation Center ofChemical Science and Engineering(Tianjin),Tianjin 300072,China;Joint School of National University of Singapore andTianjin University,International Campus of Tianjin University, Binhai New City,Fuzhou 350207,China
文献出处：
引用格式：
[1]Guangyi Jiang;Daliang Han;Zishan Han;Jiachen Gao;Xinyu Wang;Zhe Weng;Quan-Hong Yang-.Rational Manipulation of Intermediates on Copper for CO2 Electroreduction Toward Multicarbon Products)[J].天津大学学报（英文版）,2022(04):265-291
A类：
Intermediates,Multicarbon
B类：
Rational,Manipulation,Copper,Electroreduction,Toward,Products,Excess,greenhouse,gas,emissions,primarily,dioxide,have,caused,major,environmental,concerns,worldwide,electroreduction,into,valuable,chemicals,using,renewable,energy,ecofriendly,approach,achieve,neutrality,this,regard,copper,has,attracted,considerable,attention,only,known,metallic,available,converting,high,value,multicarbon,2+,products,production,involves,complicated,coupling,steps,thus,imposes,demands,regulation,review,we,discuss,multiple,strategies,modulating,intermediates,facilitate,formation,catalysts,Furthermore,several,sophisticated,insitu,characterization,techniques,are,outlined,elucidating,mechanism,Lastly,challenges,future,directions,envisioned
AB值：
0.720033
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