典型文献
A facile path from fast synthesis of Li-argyrodite conductor to dry forming ultrathin electrolyte membrane for high-energy-density all-solid-state lithium batteries
文献摘要：
All-solid-state lithium batteries(ASSLBs),utilizing sulfide solid electrolyte,are considered as the promis-ing design on account of their superior safety and high energy density,whereas the time-consuming preparation process of sulfide electrolyte powders and the thickness of electrolyte layer hinder their practical application.Herein,an innovative ultimate-energy mechanical alloying plus rapid thermal pro-cessing approach is employed to rapidly synthesize the crystalline Argyrodite-type conductor Li5.3PS4.3ClBr0.7(LPSClBr)with superior ionic conductivity(11.7 mS cm-1).Furthermore,to realize the higher energy density of the battery,an ultrathin LPSClBr sulfide electrolyte membrane with superior ionic conductivity of 6.5 mS cm-1 is fabricated with the aid of polytetrafluoroethylene(PTFE)binder and the reinforced cellulose mesh.Moreover,a simple solid electrolyte interphase(SEI)is constructed on the surface of lithium metal to enhance anodic stability.Benefiting from the joint efforts of these mer-its,the modified ASSLBs with a high cell-level energy density of 311 Wh kg-1 show an excellent cyclic stability.The assembled all-solid-state Li2S/Li pouch cell can operate even under the severe conditions of bending and cutting,demonstrating the enormous potential of the sulfide electrolyte membrane for ASSLBs application.
文献关键词：
中图分类号：
作者姓名：
Zhao Jiang;Hongling Peng;Jingru Li;Yu Liu;Yu Zhong;Changdong Gu;Xiuli Wang;Xinhui Xia;Jiangping Tu
作者机构：
State Key Laboratory of Silicon Materials,Key Laboratory of Advanced Materials and Applications for Batteries of Zhejiang Province,and School of Materials Science and Engineering,Zhejiang University,Hangzhou 310027,Zhejiang,China;CCTEG Chongqing Research Institute,Chongqing 400039,China
文献出处：
引用格式：
[1]Zhao Jiang;Hongling Peng;Jingru Li;Yu Liu;Yu Zhong;Changdong Gu;Xiuli Wang;Xinhui Xia;Jiangping Tu-.A facile path from fast synthesis of Li-argyrodite conductor to dry forming ultrathin electrolyte membrane for high-energy-density all-solid-state lithium batteries)[J].能源化学,2022(11):309-316
A类：
Argyrodite,3PS4,3ClBr0,LPSClBr
B类：
facile,path,from,fast,synthesis,argyrodite,conductor,dry,forming,ultrathin,electrolyte,membrane,energy,density,solid,state,lithium,batteries,All,ASSLBs,utilizing,sulfide,are,considered,promis,design,account,their,superior,safety,whereas,consuming,preparation,process,powders,thickness,layer,hinder,practical,application,Herein,innovative,ultimate,mechanical,alloying,plus,thermal,cessing,approach,employed,rapidly,synthesize,crystalline,type,Li5,ionic,conductivity,mS,Furthermore,realize,higher,battery,fabricated,aid,polytetrafluoroethylene,PTFE,binder,reinforced,cellulose,mesh,Moreover,simple,interphase,SEI,constructed,surface,metal,enhance,anodic,stability,Benefiting,joint,efforts,these,mer,its,modified,level,Wh,show,excellent,cyclic,assembled,Li2S,pouch,can,operate,even,under,severe,conditions,bending,cutting,demonstrating,enormous,potential
AB值：
0.567398
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机标中图分类号，由域田数据科技根据网络公开资料自动分析生成，仅供学习研究参考。
