典型文献
Crystal facet-dependent electrocatalytic performance of metallic Cu in CO2 reduction reactions
文献摘要：
Developing high-performance electrocatalysts for CO2 reduction reaction(CO2RR)is crucial since it is beneficial for environmental protection and the resulting value-add chemical products can act as an al-ternative to fossil feedstocks.Nonetheless,the direct reduction of CO2 into long-chain hydrocarbons and oxygenated hydrocarbons with high selectivity remains challenging.Copper(Cu)shows a distinctive ad-vantage that it is the only pure metal catalyst for reducing CO2 into multi-carbon(C2+)products and the certain facets(e.g.,(100),(111),(111))of Cu nanocrystals exhibit relatively low energy barriers for the formation of specific products(e.g.,CO,HCOOH,CH4,C2H4,C2H5OH,and other C2+products).Therefore,extensive studies have been carried out to explore the relationship between the facets of Cu nanocrystals and corresponding catalytic products.In this review,we will discuss the crystal facet-dependent electro-catalytic CO2RR performance in metallic Cu catalysts,meanwhile,the detailed reaction mechanisms will be systematically summarized.In addition,we will provide a personal perspective for the future research directions in this emerging field.We believe this review is helpful to guide the design of high-selectivity Cu-based electrocatalysts for CO2RR.
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作者姓名：
Hao Zhang;Caihong He;Sumei Han;Zeyang Du;Ling Wang;Qinbai Yun;Wenbin Cao;Bowei Zhang;Ya-Hui Tian;Qipeng Lu
作者机构：
School of Materials Science and Engineering,University of Science and Technology Beijing,Beijing 100083,China;Department of Chemistry,City University of Hong Kong,Hong Kong,China;Institute for Advanced Materials and Technology,University of Science and Technology Beijing,Beijing 100083,China;Institute of Acoustics,Chinese Academy of Sciences,Beijing 10019,China
文献出处：
引用格式：
[1]Hao Zhang;Caihong He;Sumei Han;Zeyang Du;Ling Wang;Qinbai Yun;Wenbin Cao;Bowei Zhang;Ya-Hui Tian;Qipeng Lu-.Crystal facet-dependent electrocatalytic performance of metallic Cu in CO2 reduction reactions)[J].中国化学快报（英文版）,2022(08):3641-3649
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0.555817
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