典型文献
Rational catalyst design and interface engineering for electrochemical CO2 reduction to high-valued alcohols
文献摘要：
Electrochemical CO2 reduction(eCO2RR)is an emerging strategy to address the global carbon balance issues and fulfill the carbon-neutral goal through converting CO2 to value-added chemicals/fuels driven by renewable energy sources.The production of highly reduced carbon compounds beyond CO and for-mate,especially oxygenate alcohol products with high energy densities and large global market capaci-ties,is particularly desirable for practical applications.However,the building of alcohol-selective eCO2RR electrocatalysis systems to overcome the high overpotential and poor durability remains a big challenge.Recently,diverse strategies have been developed for rational catalyst design towards alcohol productions from eCO2RR on the basis of the corresponding reaction mechanisms.In this review article,we firstly highlight recent advances in fundamental understanding of mechanisms in three electrochemical CO2-alcohol reaction pathways.Then,the design strategies focused on catalyst and interface design are sum-marized for building alcohol-selective eCO2RR electrocatalysis systems.The advanced characterization techniques are also discussed to provide more insights into eCO2RR-to-alcohols processes.Finally,the remaining challenges and perspectives for promoting eCO2RR to alcohols are proposed.
文献关键词：
中图分类号：
作者姓名：
Lingxi Zhou;Ruitao Lv
作者机构：
State Key Laboratory of New Ceramics and Fine Processing,School of Materials Science and Engineering,Tsinghua University,Beijing 100084,China;Key Laboratory of Advanced Materials(MOE),School of Materials Science and Engineering,Tsinghua University,Beijing 100084,China
文献出处：
引用格式：
[1]Lingxi Zhou;Ruitao Lv-.Rational catalyst design and interface engineering for electrochemical CO2 reduction to high-valued alcohols)[J].能源化学,2022(07):310-331
A类：
eCO2RR,oxygenate
B类：
Rational,catalyst,design,interface,engineering,electrochemical,reduction,valued,alcohols,Electrochemical,emerging,strategy,address,global,carbon,balance,issues,fulfill,neutral,goal,through,converting,added,chemicals,fuels,driven,by,renewable,energy,sources,highly,reduced,compounds,beyond,mate,especially,products,densities,large,market,capaci,particularly,desirable,practical,applications,However,building,selective,electrocatalysis,systems,overcome,overpotential,poor,durability,remains,big,Recently,diverse,strategies,have,been,developed,rational,towards,productions,from,basis,corresponding,reaction,mechanisms,In,this,review,article,firstly,highlight,recent,advances,fundamental,understanding,three,pathways,Then,focused,are,sum,marized,advanced,characterization,techniques,also,discussed,provide,more,insights,into,processes,Finally,remaining,challenges,perspectives,promoting,proposed
AB值：
0.587552
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