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典型文献
Research progress of precise structural regulation of single atom catalyst for accelerating electrocatalytic oxygen reduction reaction
文献摘要:
The development and utilization of renewable clean energy can effectively solve the two major problems of energy and environment.As an efficient power generation device that converts hydrogen energy into elec-tric energy,fuel cell has attracted more and more attention.For fuel cells,the oxygen reduction reaction(ORR)at the cathode is the core reaction,and the design and development of high-performance ORR cata-lysts remain quite challenging.Since the microenvironment of the active center of single atom catalysts(SACs)has an important influence on its catalytic performance,it has been a research focus to improve the ORR activity and stability of electrocatalysts by adjusting the structure of the active center through rea-sonable structural regulation methods.In this review,we reviewed the preparation and structure-activity relationship of SACs for ORR.Then,the structural precision regulation methods for improving the activity and stability of ORR electrocatalysts are discussed.And the advanced in-situ characterization techniques for revealing the changes of active sites in the electrocatalytic ORR process are summarized.Finally,the chal-lenges and future design directions of SACs for ORR are discussed.This work will provide important refer-ence value for the design and synthesis of SACs with high activity and stability for ORR.
文献关键词:
作者姓名:
Minmin Wang;Hui Zhang;Yunqi Liu;Yuan Pan
作者机构:
State Key Laboratory of Heavy Oil Processing,China University of Petroleum(East China),Qingdao 266580,Shandong,China
文献出处:
引用格式:
[1]Minmin Wang;Hui Zhang;Yunqi Liu;Yuan Pan-.Research progress of precise structural regulation of single atom catalyst for accelerating electrocatalytic oxygen reduction reaction)[J].能源化学,2022(09):56-72
A类:
sonable
B类:
Research,progress,precise,structural,regulation,single,atom,accelerating,electrocatalytic,oxygen,reduction,reaction,development,utilization,renewable,clean,energy,can,effectively,solve,two,major,problems,efficient,power,generation,device,that,converts,hydrogen,into,tric,fuel,has,attracted,more,attention,For,cells,ORR,cathode,core,design,high,performance,remain,quite,challenging,Since,microenvironment,active,center,SACs,important,influence,its,been,research,focus,improve,activity,stability,electrocatalysts,by,adjusting,structure,through,methods,In,this,reviewed,preparation,relationship,Then,precision,improving,are,discussed,And,advanced,situ,characterization,techniques,revealing,changes,sites,process,summarized,Finally,lenges,future,directions,This,work,will,provide,refer,value,synthesis
AB值:
0.508201
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