典型文献
Rational design strategies of Cu-based electrocatalysts for CO2 electroreduction to C2 products
文献摘要：
Electrochemical reduction of CO2(CO2RR)to high value-added chemicals is an effective way to remove excess CO2 from the atmosphere.Due to the unique propensity of Cu for valuable hydrocarbons,Cu-based electrocatalysts are the most potential catalysts that allow the conversion of CO2 into a variety of C2 products such as ethylene and ethanol.Rational design of Cu-based catalysts can improve their directional selectivity to C2 products.Hence,in this review,we summarize the recent progress in the mechanistic studies of Cu-based catalysts on reducing CO2 to C2 products.We focus on three key strate-gies for efficiently enhancing electrocatalytic performance of Cu-based catalysts,including tuning elec-tronic structure,surface structure,and coordination environment.The correlation between the structural characteristics of Cu-based catalysts and their activity and selectivity to C2 products is dis-cussed.Finally,we discuss the challenges in the field of CO2 electroreduction to C2 products and provide the perspectives to design efficient Cu-based catalysts in the future.
文献关键词：
中图分类号：
作者姓名：
Shuo Liu;Baoshan Zhang;Lihong Zhang;Jie Sun
作者机构：
Key Laboratory for Green Chemical Technology of Ministry of Education,School of Chemical Engineering and Technology,Tianjin University,Tianjin 300072,China;School of Chemical Engineering and Technology,Tianjin University,Tianjin 300072,China
文献出处：
引用格式：
[1]Shuo Liu;Baoshan Zhang;Lihong Zhang;Jie Sun-.Rational design strategies of Cu-based electrocatalysts for CO2 electroreduction to C2 products)[J].能源化学,2022(08):63-82
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Rational,design,strategies,electrocatalysts,electroreduction,C2,products,Electrochemical,CO2RR,high,value,added,chemicals,effective,way,remove,excess,from,atmosphere,Due,unique,propensity,valuable,hydrocarbons,are,most,potential,that,allow,conversion,into,variety,such,ethylene,ethanol,can,improve,their,directional,selectivity,Hence,this,review,summarize,recent,progress,mechanistic,studies,reducing,We,focus,three,key,efficiently,enhancing,electrocatalytic,performance,including,tuning,tronic,structure,surface,coordination,environment,correlation,between,structural,characteristics,activity,cussed,Finally,discuss,challenges,field,provide,perspectives,future
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0.531397
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