典型文献
Beyond catalytic materials:Controlling local gas/liquid environment in the catalyst layer for CO2 electrolysis
文献摘要：
Electrochemical reduction of CO2 to value-added chemicals using renewable electricity provides a promising strategy to achieve sustainable fuel production and carbon neutrality.Along with the develop-ment of electrocatalysts,flow cells with gas-diffusion electrodes(GDEs)have been used to reach com-mercially viable current densities for CO2 electrolysis,while the local environment and CO2 mass transport in the electrodes remain to be elucidated.In this review article,we highlight some insights into the microenvironment in the catalyst layer for CO2 electrolysis,including typical mass transport models for CO2 reduction in H-type cells and GDE flow cells,the effect of a hydrophobic microenvironment on CO2 mass transport and catalytic performance,and the formation of a gas/liquid balance and solid-liq-uid-gas interfaces for CO2 electrolysis.The insights and discussions in this article can provide important guidelines on the design of catalysts,electrodes,and electrolyzers for CO2 electrolysis,as well as other gas-involving electrocatalytic reactions.
文献关键词：
中图分类号：
作者姓名：
Zhuo Xing;Kaige Shi;Xun Hu;Xiaofeng Feng
作者机构：
School of Material Science and Engineering,University of Jinan,Jinan 250022,Shandong,China;Department of Physics,University of Central Florida,Orlando,FL 32816,United States;Renewable Energy and Chemical Transformations(REACT)Cluster,University of Central Florida,Orlando,FL 32816,United States
文献出处：
引用格式：
[1]Zhuo Xing;Kaige Shi;Xun Hu;Xiaofeng Feng-.Beyond catalytic materials:Controlling local gas/liquid environment in the catalyst layer for CO2 electrolysis)[J].能源化学,2022(03):45-51
A类：
GDEs
B类：
Beyond,materials,Controlling,local,gas,liquid,layer,electrolysis,Electrochemical,reduction,value,added,chemicals,using,renewable,electricity,provides,promising,strategy,achieve,sustainable,fuel,production,carbon,neutrality,Along,develop,electrocatalysts,flow,cells,diffusion,electrodes,have,been,used,reach,com,mercially,viable,current,densities,while,mass,transport,remain,elucidated,In,this,review,article,highlight,some,insights,into,microenvironment,including,typical,models,type,effect,hydrophobic,performance,formation,balance,solid,interfaces,discussions,can,important,guidelines,design,electrolyzers,well,other,involving,electrocatalytic,reactions
AB值：
0.53246
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