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典型文献
Attaining enhanced thermoelectric performance in p-type(SnSe)1-x(SnS2)x produced via sintering their solution-synthesized micro/nanostructures
文献摘要:
SnSe,possessing strong lattice anharmonicity and structural anisotropy,has attracted massive attention in thermoelectric conversion.Herein,we demonstrate that simultaneously optimized electrical and ther-mal transport properties are achieved in SnS2-alloyed SnSe polycrystalline materials,which were fabri-cated via sintering the mixture of solution-synthesized SnSe microplates and SnS2 nanoplates.Resulting from the increased carrier concentration,p-type(SnSe)1-x(SnS2)x(x = 0.5%,1%)samples obtain much-improved power factor between 300 K and 373 K,e.g.0.72 mW m-1 K-2 at 300 K for(SnSe)0.99(SnS2)0.01,which is enhanced by 53%compared to that of SnSe.Additionally,the existing point defects and planar defects effectively strengthen phonon scattering,thus reducing the lattice thermal conductivity,for ex-ample,0.47 W m-1 K-1 at 773 K for the x = 0.02 sample.Eventually,a maximum zT of 0.80 at 823 K and an average zT of 0.52 over 300-823 K are obtained in the(SnSe)0.99(SnS2)0.01 sample,which are increased by 33%and 45%compared to those of SnSe,respectively.This study demonstrates a secondary phase alloying strategy to synergistically optimize the electrical and thermal properties of polycrystalline SnSe.
文献关键词:
作者姓名:
Xiaofang Liu;Hengyang Wang;Bin Zhang;Sikang Zheng;Yao Chen;Hong Zhang;Xianhua Chen;Guoyu Wang;Xiaoyuan Zhou;Guang Han
作者机构:
College of Materials Science and Engineering,Chongqing University,Chongqing,400044,China;National Engineering Research Center for Magnesium Alloys,Chongqing University,Chongqing,400044,China;Analytical and Testing Center,Chongqing University,Chongqing,401331,China;College of Physics,Chongqing University,Chongqing,401331,China;Chongqing Institute of Green and Intelligent Technology,Chinese Academy of Sciences,Chongqing,400714,China
引用格式:
[1]Xiaofang Liu;Hengyang Wang;Bin Zhang;Sikang Zheng;Yao Chen;Hong Zhang;Xianhua Chen;Guoyu Wang;Xiaoyuan Zhou;Guang Han-.Attaining enhanced thermoelectric performance in p-type(SnSe)1-x(SnS2)x produced via sintering their solution-synthesized micro/nanostructures)[J].材料科学技术(英文版),2022(25):205-213
A类:
Attaining,Resulting
B类:
enhanced,thermoelectric,performance,type,SnSe,SnS2,produced,via,sintering,their,solution,synthesized,nanostructures,possessing,strong,lattice,anharmonicity,structural,anisotropy,attracted,massive,attention,conversion,Herein,that,simultaneously,optimized,electrical,transport,properties,achieved,alloyed,polycrystalline,materials,which,were,fabri,cated,mixture,microplates,nanoplates,from,increased,carrier,concentration,samples,much,improved,power,between,mW,by,compared,Additionally,existing,point,defects,planar,effectively,strengthen,phonon,scattering,thus,reducing,thermal,conductivity,Eventually,maximum,zT,average,over,obtained,those,respectively,This,study,demonstrates,secondary,phase,alloying,strategy,synergistically
AB值:
0.518376
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