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典型文献
Gas-liquid-liquid slug flow and mass transfer in hydrophilic and hydrophobic microreactors
文献摘要:
Gas-liquid-liquid three-phase slug flow was generated in both hydrophilic and hydrophobic microreac-tors with double T-junctions.The bubble-droplet relative movement and the local mass transfer within the continuous slug and the dispersed droplet were investigated.It was found that bubbles moved faster than droplets under low capillary number(Ca),while droplets moved faster upon the increase of Ca due to the increased inertia.For the first time,we observed that the increased viscosity of droplets fastened the droplet movement.The mass transfer in the continuous slug was dominated by convection,leading to nearly constant global mass transfer coefficient(kLa);while that in the dispersed droplet was dominated by diffusion,resulting in kL decreasing along the channel.Such features are analogical to the correspond-ing gas-liquid or liquid-liquid two-phase slug flow,but the formation of bubble-droplet clusters caused by relative movement lowered the absolute mass transfer coefficient.These results provide insights for the precise manipulation of gas-liquid-liquid slug flow in microreactors towards process optimization.
文献关键词:
作者姓名:
Yanyan Liu;Chaoqun Yao;Guangwen Chen
作者机构:
Dalian National Laboratory for Clean Energy,Dalian Institute of Chemical Physics,Chinese Academy of Sciences,Dalian 116023,China;University of Chinese Academy of Sciences,Beijing 100049,China
引用格式:
[1]Yanyan Liu;Chaoqun Yao;Guangwen Chen-.Gas-liquid-liquid slug flow and mass transfer in hydrophilic and hydrophobic microreactors)[J].中国化学工程学报(英文版),2022(10):85-94
A类:
microreac,fastened
B类:
Gas,liquid,slug,flow,mass,transfer,hydrophilic,hydrophobic,microreactors,three,phase,was,generated,both,double,junctions,relative,movement,local,within,continuous,dispersed,investigated,It,found,that,bubbles,moved,faster,than,droplets,under,capillary,number,while,upon,due,increased,inertia,For,first,observed,viscosity,dominated,by,convection,leading,nearly,constant,global,coefficient,kLa,diffusion,resulting,decreasing,along,channel,Such,features,are,analogical,correspond,gas,two,but,formation,clusters,caused,lowered,absolute,These,results,provide,insights,precise,manipulation,towards,process,optimization
AB值:
0.467655
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