典型文献
Insightful understanding of three-phase interface behaviors in 1T-2H MoS2/CFP electrode for hydrogen evolution improvement
文献摘要：
Hydrogen evolution reaction(HER)catalytic electrodes under actual working conditions show interest-ing mass transfer behaviors at solid(electrode)/liquid(electrolyte)/gas(hydrogen)three-phase interfaces.These behaviors are essential for forming a continuous and effective physical contact region between the electrolyte and the electrode and require further detailed understanding.Here,a case study on 1T-2H phase molybdenum disulfide(MoS2)/carbon fiber paper(CFP)catalytic electrodes is performed.Rapid gas-liquid mass transfer at the interface for enhancing the working area stability and capillarity for in-creasing the electrode working area is found.The real scenario,wherein the energy utilization efficiency of the as-prepared non-noble metal catalytic electrode exceeds that of the noble metal catalytic electrode,is disclosed.Specifically,a fluid dynamics model is developed to investigate the behavior mechanism of hydrogen bubbles from generation to desorption on the catalytic electrode surface with different hy-drophilic and hydrophobic properties.These new insights and theoretical evidence on the non-negligible three-phase interface behaviors will identify opportunities and motivate future research in high-efficiency,stability,and low-cost HER catalytic electrode development.
文献关键词：
中图分类号：
作者姓名：
Jiamu Cao;Jing Zhou;Mingxue Li;Junyu Chen;Yufeng Zhang;Xiaowei Liu
作者机构：
School of Astronautics,Harbin Institute of Technology,Harbin 150001,China;MEMS Center,Harbin Institute of Technology,Harbin 150001,China;Key Laboratory of Micro-systems and Micro-structures Manufacturing.Ministry of Education,Harbin 150001,China
文献出处：
引用格式：
[1]Jiamu Cao;Jing Zhou;Mingxue Li;Junyu Chen;Yufeng Zhang;Xiaowei Liu-.Insightful understanding of three-phase interface behaviors in 1T-2H MoS2/CFP electrode for hydrogen evolution improvement)[J].中国化学快报（英文版）,2022(08):3745-3751
A类：
Insightful,drophilic
B类：
understanding,three,phase,behaviors,1T,2H,MoS2,CFP,hydrogen,evolution,improvement,Hydrogen,reaction,HER,catalytic,electrodes,actual,working,conditions,show,interest,mass,transfer,solid,liquid,electrolyte,gas,interfaces,These,essential,forming,continuous,effective,physical,contact,region,between,require,further,detailed,Here,case,study,molybdenum,disulfide,carbon,fiber,paper,performed,Rapid,enhancing,area,stability,capillarity,creasing,found,real,scenario,wherein,energy,utilization,efficiency,prepared,noble,metal,exceeds,that,disclosed,Specifically,fluid,dynamics,model,developed,investigate,mechanism,bubbles,from,generation,desorption,surface,different,hydrophobic,properties,new,insights,theoretical,evidence,negligible,will,identify,opportunities,motivate,future,research,high,low,cost,development
AB值：
0.544807
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