典型文献
Alcohol-assisted hydrodeoxygenation as a sustainable and cost-effective pathway for biomass derivatives upgrading
文献摘要：
Hydrodeoxygenation(HDO)is one of the most promising strategies for the upgrading of biomass-derived compounds to chemicals and fuels.However,the conventional HDO process accompanied by insecure high-pressure H2 leads to the hefty infrastructure cost on the industrial scale and inevitably trigger over-all hydrogenation which is considered as an uncontrollable and risky approach.Accordingly,the devel-opments of alcohol-assisted HDO can be viewed as a sustainable and cost-effective alternative.This review critically summarizes the potentials and challenges of alcohol-assisted strategy from diverse per-spectives including safety,economics and catalytic efficiency.Based on the discrepancies of in-situ hydrogen generation,the alcohol-assisted strategy is divided into combined reforming-HDO route and catalytic transfer hydrogenation/hydrogenolysis(CTH)route.Furthermore,describe different catalytic behaviors and elaborate their applications among several upgrading processes of representative biomass model compounds,aiming to illustrate their potentials in biomass utilization.The influence of alcohols is highlighted because they act both hydrogen donor and solvent.At last,the current challenges and per-spectives of alcohol-assisted HDO are proposed for further development and improvement.
文献关键词：
中图分类号：
作者姓名：
Hao Xu;Hao Li
作者机构：
National-Local Joint Engineering Laboratory for Energy Conservation in Chemical Process Integration and Resources Utilization,Tianjin Key Laboratory of Chemical Process Safety,School of Chemical Engineering and Technology,Hebei University of Technology,Tianjin 300130,China
文献出处：
引用格式：
[1]Hao Xu;Hao Li-.Alcohol-assisted hydrodeoxygenation as a sustainable and cost-effective pathway for biomass derivatives upgrading)[J].能源化学,2022(10):133-159
A类：
Hydrodeoxygenation,hefty
B类：
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AB值：
0.605653
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