典型文献
Carbon-based single atom catalyst:Synthesis,characterization,DFT calculations
文献摘要:
Carbon-based single-atom catalysts(SACs)with atomic sizes of active sites have become the promising candidates for a variety of catalytic systems because of their high atom utilization,and unique electronic structures.Different types of single-atom sites can be fabricated via multiple preparation strategies,which would demonstrate distinct different coordination configurations and electronic features,and ultimately affected the structure-catalysis relationship of SACs in targeted reactions.As a result,it is necessary to identify the active sites of SACs and understand the structure-catalysis relationship of SACs at the atomic scale.In this review,a variety of preparation strategies of carbon-based SACs were documented.Then,the recent development on versatile characterization techniques and computational achievements were sum-marized regarding in understanding the electronic and geometric characteristics of carbon-based SACs.Finally,major challenges and development directions concerning single-atom sites identification and ad-vanced tools development are discussed to shed light on future research of carbon-based SACs.
文献关键词:
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作者姓名:
Yanan Shang;Xiaoguang Duan;Shaobin Wang;Qinyan Yue;Baoyu Gao;Xing Xu
作者机构:
Shandong Key Laboratory of Water Pollution Control and Resource Reuse,School of Environmental Science and Engineering,Shandong University,Ji'nan 250100,China;School of Chemical Engineering and Advanced Materials,The University of Adelaide,Adelaide,SA 5005,Australia
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引用格式:
[1]Yanan Shang;Xiaoguang Duan;Shaobin Wang;Qinyan Yue;Baoyu Gao;Xing Xu-.Carbon-based single atom catalyst:Synthesis,characterization,DFT calculations)[J].中国化学快报(英文版),2022(02):663-673
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0.57882
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