典型文献
2D materials for solar fuels via artificial photosynthesis
文献摘要:
To create a globally carbon neutral so-ciety,sustainable energy systems to re-place fossil fuels are needed urgently.Photosynthesis in nature converts CO2 and H2O into carbohydrates and O2 and is driven by solar energy via pho-tosystem Ⅱ(PSⅡ)and photosystem Ⅰ(PSⅠ)[1].Water oxidation occurring at the oxygen-evolution complex(OEC:CaMn4O5)of PSⅡ is the primary source of protons and electrons for the reduc-tion of CO2 by Ribulose-1,5-biphosphate carboxylate/oxygenase(RuBisCo).The protons and electrons produced in PSⅡare also utilized directly or indirectly in other enzyme catalysis reactions such as the H2 evolution reaction(HER)by hy-drogenases(H2ase),N2-fixing reaction by nitrogenase(N2ase)or O2 reduction reaction by cytochrome c oxidase(CCO)(Fig.1).Inspired by the function of pho-tosynthesis,chemical processes includ-ing water splitting,CO2 reduction and N2 fixation can be replicated via artificial photosynthesis(AP).
文献关键词:
中图分类号:
作者姓名:
Jian Du;Hao Yang;Licheng Sun
作者机构:
Institute of Natural Sciences,Westlake Institute for Advanced Study,China;Center of Artificial Photosynthesis for Solar Fuels,School of Science,Westlake University,China;Department of Chemistry,School of Engineering Sciences in Chemistry,Biotechnology and Health,KTH Royal Institute of Technology,Sweden;State Key Laboratory of Fine Chemicals,DUT-KTH Joint Education and Research Centre on Molecular Devices,Dalian University of Technology,China
文献出处:
引用格式:
[1]Jian Du;Hao Yang;Licheng Sun-.2D materials for solar fuels via artificial photosynthesis)[J].国家科学评论(英文版),2022(05):14-16
A类:
tosystem,CaMn4O5,Ribulose,biphosphate,RuBisCo,drogenases,H2ase,N2ase
B类:
2D,materials,solar,fuels,via,artificial,photosynthesis,To,create,globally,carbon,neutral,ciety,sustainable,energy,systems,place,fossil,are,needed,urgently,Photosynthesis,nature,converts,H2O,into,carbohydrates,driven,by,PS,photosystem,Water,oxidation,occurring,evolution,complex,OEC,primary,source,protons,electrons,carboxylate,oxygenase,produced,also,utilized,indirectly,other,enzyme,catalysis,reactions,such,HER,fixing,nitrogenase,reduction,cytochrome,oxidase,CCO,Fig,Inspired,function,chemical,processes,includ,water,splitting,fixation,can,be,replicated,AP
AB值:
0.532106
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