典型文献
Selective Oxidation of Methane into Methanol Under Mild Conditions
文献摘要：
S elective oxidation of methane to methanol under mild conditions has been considered as a dream reaction but suffers from poor efficiency due to the strong C—H bond of methane and easy overoxidation of the methanol product.For overcoming these problems,a series of strategies has been developed for improving methanol productivity with oxidants of hydrogen peroxide and even a mixture of oxygen and hydrogen at mild temperatures.Significant achievements in these strategies using effective catalysts,such as supported metal nanoparticles,colloidal metal nanoparticles,and metal@zeolites are briefly concluded.Moreover,the current challenges,future perspectives for preparing active,selective,and stable catalysts,have been discussed.The zeolite fixed metal nanoparticle structure has been found to boost the reaction by benefiting the formation and enrichment of peroxide intermediates,which might guide the development of more efficient catalysts.
文献关键词：
中图分类号：
作者姓名：
LIU Yifeng;WANG Liang;XIAO Feng-Shou
作者机构：
Key Lab of Applied Chemistry of Zhejiang Province,Department of Chemistry,Zhejiang University,Hangzhou 310028,P.R.China;Key Lab of Biomass Chemical Engineering of Ministry of Education,College of Chemical and Biological Engineering,Zhejiang University,Hang-zhou 310027,P.R.China;Zhejiang Tianlan Environmental Protection Technology Limited Company,Hangzhou 310012,P.R.China
文献出处：
引用格式：
[1]LIU Yifeng;WANG Liang;XIAO Feng-Shou-.Selective Oxidation of Methane into Methanol Under Mild Conditions)[J].高等学校化学研究（英文版）,2022(03):671-676
A类：
overoxidation
B类：
Selective,Oxidation,Methane,into,Methanol,Under,Mild,Conditions,methane,methanol,under,mild,conditions,has,been,considered,dream,reaction,but,suffers,from,poor,efficiency,due,strong,bond,easy,For,overcoming,these,problems,series,strategies,developed,improving,productivity,oxidants,hydrogen,peroxide,even,mixture,oxygen,temperatures,Significant,achievements,using,effective,catalysts,such,supported,metal,nanoparticles,colloidal,zeolites,are,briefly,concluded,Moreover,current,challenges,future,perspectives,preparing,active,selective,stable,have,discussed,fixed,structure,found,boost,by,benefiting,formation,enrichment,intermediates,which,might,guide,development,more,efficient
AB值：
0.665212
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