典型文献
Molecular-level Engineering of S-scheme Heterojunction: the Site-specific Role for Directional Charge Transfer
文献摘要:
The promising S-scheme heterojunction photocatalysts are considered as a novel frontier due to their superiority in various solar-driven energy-related applications. Recently, a novel atom-specific tailoring strategy has been introduced on the construction of S-scheme heterojunction for promoting the electronic transferability. The S-scheme heterojunction is regulated by integrating high-crystalline carbon nitride with Co-doped CeO2. Specifically, this atom-specific regulation of S-scheme heterojunction boosts directional electron-driving effect towards functionalized Co sites, benefit-ing for effective photogenerated charge carrier transferability. Moreover, a series of tracking characterizations show that Co-embedded modification promotes CO2 photoreduction into hydrogenation steps, resulting in high performance towards CO2-to-CH4 photoreduction, which provides new opportunities for the development of multifunctional cooperation in heterogeneous photocatalysis.
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作者姓名:
Jianjun Zhang;Linxi Wang;Mitra Mousavi;Jahan B.Ghasemi;Jiaguo Yu
作者机构:
Laboratory of Solar Fuel,Faculty of Materials Science and Chemistry,China University of Geosciences,Wuhan 430074,China;School of Chemistry,College of Science,University of Tehran,P.O.Box 14155-6455,Tehran,Iran
文献出处:
引用格式:
[1]Jianjun Zhang;Linxi Wang;Mitra Mousavi;Jahan B.Ghasemi;Jiaguo Yu-.Molecular-level Engineering of S-scheme Heterojunction: the Site-specific Role for Directional Charge Transfer)[J].结构化学,2022(06):3-5
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Molecular,level,Engineering,scheme,Heterojunction,Site,specific,Role,Directional,Charge,Transfer,promising,heterojunction,photocatalysts,are,considered,novel,frontier,due,their,superiority,various,solar,driven,energy,related,applications,Recently,atom,tailoring,strategy,has,been,introduced,construction,promoting,electronic,transferability,regulated,by,integrating,high,crystalline,carbon,nitride,Co,doped,CeO2,Specifically,this,regulation,boosts,directional,driving,towards,functionalized,sites,benefit,effective,photogenerated,charge,carrier,Moreover,series,tracking,characterizations,show,that,embedded,modification,promotes,photoreduction,into,hydrogenation,steps,resulting,performance,CH4,which,provides,new,opportunities,development,multifunctional,cooperation,heterogeneous,photocatalysis
AB值:
0.732058
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