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典型文献
The mechanism study of low-pressure air plasma cleaning on large-aperture optical surface unraveled by experiment and reactive molecular dynamics simulation
文献摘要:
Low-pressure air plasma cleaning is an effective method for removing organic contaminants on large-aperture optical components in situ in the inertial confinement fusion facility.Chemical reactions play a significant role in plasma cleaning,which is a complex process involving abundant bond cleavage and species generation.In this work,experiments and reactive molecular dynamics simulations were carried out to unravel the reaction mechanism between the benchmark organic contaminants of dibutyl phthalate and air plasma.The optical emission spectroscopy was used to study the overall evolution behaviors of excited molecular species and radical signals from air plasma as a reference to simulations.Detailed reaction pathways were revealed and characterized,and specific intermediate radicals and products were analyzed during experiments and simulation.The reactive species in the air plasma,such as O,HO2 and O3 radicals,played a crucial role in cleaving organic molecular structures.Together,our findings provide an atomic-level understanding of complex reaction processes of low-pressure air plasma cleaning mechanisms and are essential for its application in industrial plasma cleaning.
文献关键词:
作者姓名:
Yuhai LI;Qingshun BAI;Yuheng GUAN;Hao LIU;Peng ZHANG;Buerlike BATELIBIEKE;Rongqi SHEN;Lihua LU;Xiaodong YUAN;Xinxiang MIAO;Wei HAN;Caizhen YAO
作者机构:
School of Mechatronics Engineering,Harbin Institute of Technology,Harbin 150000,People's Republic of China;Research Center of Laser Fusion,China Academy of Engineering Physics,Mianyang 621900,People's Republic of China;Chongqing Research Institute,Harbin Institute of Technology,Chongqing 401135,People's Republic of China
引用格式:
[1]Yuhai LI;Qingshun BAI;Yuheng GUAN;Hao LIU;Peng ZHANG;Buerlike BATELIBIEKE;Rongqi SHEN;Lihua LU;Xiaodong YUAN;Xinxiang MIAO;Wei HAN;Caizhen YAO-.The mechanism study of low-pressure air plasma cleaning on large-aperture optical surface unraveled by experiment and reactive molecular dynamics simulation)[J].等离子体科学和技术(英文版),2022(06):77-87
A类:
B类:
study,low,pressure,air,plasma,cleaning,large,aperture,optical,surface,unraveled,by,reactive,molecular,dynamics,Low,effective,method,removing,organic,contaminants,components,situ,inertial,confinement,fusion,facility,Chemical,reactions,significant,role,which,complex,involving,abundant,bond,cleavage,species,generation,In,this,work,experiments,simulations,were,carried,out,between,benchmark,dibutyl,phthalate,emission,spectroscopy,was,used,overall,evolution,behaviors,excited,signals,from,reference,Detailed,pathways,revealed,characterized,specific,intermediate,radicals,products,analyzed,during,such,HO2,O3,played,crucial,cleaving,structures,Together,our,findings,provide,atomic,level,understanding,processes,mechanisms,are,essential,its,application,industrial
AB值:
0.561384
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