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典型文献
Hierarchical porous metal-organic frameworks/polymer microparticles for enhanced catalytic degradation of organic contaminants
文献摘要:
This work reports on a simple microfluidic strategy to controllably fabricate uniform polymeric microparticles containing hierarchical porous structures integrated with highly accessible catalytic metal organic frameworks for efficient degradation of organic conta-minants.Monodisperse(W1/O)/W2 emulsion droplets generated from microfluidics are used as templates for the microparticle synthesis.The emulsion droplets contain tiny water microdroplets from homogenization and water nanodroplets from diffusion-induced swollen micelles as the dual pore-forming templates,and Fe-based metal-organic framework nanorods as the nanocatalysts.The obtained microparticles possess interconnected hierarchical porous structures decorated with highly accessible Fe-based metal-organic framework nanorods for enhanced degradation of organic contaminants via a heterogeneous Fenton-like reaction.Such a degradation performance is highlighted by using these microparticles for efficient degradation of rhodamine B in hydrogen peroxide solution.This work provides a simple and general strategy to flexib-ly combine hierarchical porous structures and catalytic metal-organic frameworks to engineer advanced micro-particles for water decontamination.
文献关键词:
作者姓名:
Ping Zhang;Yi-Han Li;Li Chen;Mao-Jie Zhang;Yang Ren;Yan-Xu Chen;Zhi Hu;Qi Wang;Wei Wang;Liang-Yin Chu
作者机构:
College of Engineering,Sichuan Normal University,Chengdu 610101,China;School of Chemical Engineering,Sichuan University,Chengdu 610065,China
引用格式:
[1]Ping Zhang;Yi-Han Li;Li Chen;Mao-Jie Zhang;Yang Ren;Yan-Xu Chen;Zhi Hu;Qi Wang;Wei Wang;Liang-Yin Chu-.Hierarchical porous metal-organic frameworks/polymer microparticles for enhanced catalytic degradation of organic contaminants)[J].化学科学与工程前沿,2022(06):939-949
A类:
conta,nanodroplets,flexib
B类:
Hierarchical,porous,metal,organic,frameworks,microparticles,enhanced,catalytic,degradation,contaminants,This,reports,simple,strategy,controllably,fabricate,uniform,polymeric,containing,hierarchical,structures,integrated,highly,accessible,efficient,Monodisperse,W1,W2,emulsion,generated,from,microfluidics,are,used,templates,synthesis,tiny,water,microdroplets,homogenization,diffusion,induced,swollen,micelles,dual,pore,forming,nanorods,nanocatalysts,obtained,possess,interconnected,decorated,via,heterogeneous,Fenton,like,reaction,Such,performance,highlighted,by,using,these,rhodamine,hydrogen,peroxide,solution,provides,general,combine,engineer,advanced,decontamination
AB值:
0.488555
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