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典型文献
3D printing interface-modified PDMS/MXene nanocomposites for stretchable conductors
文献摘要:
Additive manufacturing has rapidly evolved over recent years with the advent of polymer inks and those inks containing novel nanomaterials.The compatibility of polymer inks with nanomaterial inks remains a great challenge.Simple yet effective methods for interface improvement are highly sought-after to sig-nificantly enhance the functional and mechanical properties of printed polymer nanocomposites.In this study,we developed and modified a Ti3C2 MXene ink with a siloxane surfactant to provide compatibility with a polydimethylsiloxane(PDMS)matrix.The rheology of all the inks was investigated with parame-ters such as complex modulus and viscosity,confirming a self-supporting ink behaviour,whilst Fourier-transform infrared spectroscopy exposed the inks'reaction mechanisms.The modified MXene nanosheets have displayed strong interactions with PDMS over a wide strain amplitude.An electrical conductivity of 6.14×10-2 S cm-1 was recorded for a stretchable nanocomposite conductor containing the modified MXene ink.The nanocomposite revealed a nearly linear stress-strain relationship and a maximum stress of 0.25 MPa.Within 5%strain,the relative resistance change remained below 35%for up to 100 cycles,suggesting high flexibility,conductivity and mechanical resilience.This study creates a pathway for 3D printing conductive polymer/nanomaterial inks for multifunctional applications such as stretchable elec-tronics and sensors.
文献关键词:
作者姓名:
Mathias Aakyiir;Brayden Tanner;Pei Lay Yap;Hadi Rastin;Tran Thanh Tung;Dusan Losic;Qingshi Meng;Jun Ma
作者机构:
UniSA STEM and Future Industries Institute,University of South Australia,South Australia 5095,Australia;ARC Hub for Graphene Enabled Industry Transformation,School of Chemical Engineering and Advanced Materials,The University of Adelaide,Adelaide,South Australia 5005,Australia;Commonwealth Scientific and Industrial Research Organisation(CSIRO)Manufacturing,Clayton,Victoria 3168,Australia;College of Aerospace Engineering,Shenyang Aerospace University,Shenyang,Liaoning 110136,China
引用格式:
[1]Mathias Aakyiir;Brayden Tanner;Pei Lay Yap;Hadi Rastin;Tran Thanh Tung;Dusan Losic;Qingshi Meng;Jun Ma-.3D printing interface-modified PDMS/MXene nanocomposites for stretchable conductors)[J].材料科学技术(英文版),2022(22):174-182
A类:
B类:
printing,interface,modified,PDMS,MXene,nanocomposites,stretchable,conductors,Additive,manufacturing,has,rapidly,evolved,over,recent,years,advent,polymer,inks,those,containing,novel,nanomaterials,compatibility,remains,great,challenge,Simple,yet,effective,methods,improvement,highly,sought,after,sig,nificantly,enhance,mechanical,properties,printed,In,this,study,we,developed,Ti3C2,surfactant,provide,polydimethylsiloxane,matrix,rheology,was,investigated,parame,ters,such,complex,modulus,viscosity,confirming,self,supporting,behaviour,whilst,Fourier,transform,infrared,spectroscopy,exposed,reaction,mechanisms,nanosheets,have,displayed,strong,interactions,wide,strain,amplitude,An,electrical,conductivity,recorded,revealed,nearly,linear,stress,relationship,maximum,Within,relative,resistance,change,remained,below,cycles,suggesting,flexibility,resilience,This,creates,pathway,conductive,multifunctional,applications,tronics,sensors
AB值:
0.591192
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