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典型文献
Nearly 100%exciton utilization in highly efficient red OLEDs based on dibenzothioxanthone acceptor
文献摘要:
Improving the utilization of excitons has always been an important topic for the development of elec-troluminescence devices.In this work,we designed and synthesized three red TADF emitters TPA-DBT12,TPA-DBT3 and DTPA-DBT by employing dibenzothioxanthone(DBT)acceptor framework to stabilize the locally excited triplet state to participate in the reverse intersystem crossing(RISC)process.The fast RISC process and singlet radiation decay process gave rise to evidently enhanced exciton utilization.All of the red OLEDs based on these materials showed maximum EQE over 11%and high exciton utilization close to 100%.This work not only extend the acceptor framework for red materials but also provide a new per-spective for the design of highly efficient red TADF materials with 100%exciton utilization by managing locally excited triplet state.
文献关键词:
作者姓名:
Xiaoxiao Hu;Yuanyuan Qin;Zhiyi Li;Honglei Gao;Teng Gao;Guanhao Liu;Xiangyu Dong;Naxi Tian;Xiuxian Gu;Chun-Sing Lee;Pengfei Wang;Ying Wang
作者机构:
Key Laboratory of Photochemical Conversion and Optoelectronic Materials and CityU-CAS Joint Laboratory of Functional Materials and Devices,Technical Institute of Physics and Chemistry,Chinese Academy of Sciences,Beijing 100190,China;University of Chinese Academy of Sciences,Beijing 100049,China;Center of Super-Diamond and Advanced Films(COSDAF),City University of Hong Kong,Hong Kong,China
引用格式:
[1]Xiaoxiao Hu;Yuanyuan Qin;Zhiyi Li;Honglei Gao;Teng Gao;Guanhao Liu;Xiangyu Dong;Naxi Tian;Xiuxian Gu;Chun-Sing Lee;Pengfei Wang;Ying Wang-.Nearly 100%exciton utilization in highly efficient red OLEDs based on dibenzothioxanthone acceptor)[J].中国化学快报(英文版),2022(10):4645-4648
A类:
dibenzothioxanthone,troluminescence,DBT12,DBT3
B类:
Nearly,utilization,highly,efficient,red,OLEDs,acceptor,Improving,excitons,has,always,been,important,topic,development,elec,devices,In,this,designed,synthesized,three,TADF,emitters,DTPA,by,employing,framework,stabilize,locally,excited,triplet,state,participate,reverse,intersystem,crossing,RISC,process,fast,singlet,radiation,decay,gave,rise,evidently,enhanced,All,these,materials,showed,maximum,EQE,over,close,This,not,only,extend,but,also,provide,new,per,spective,managing
AB值:
0.513209
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