典型文献
Catalysts for electrochemical ammonia oxidation:Trend,challenge,and promise
文献摘要:
Developing sustainable and clean energy tech-nology is critial to address the current energy and environ-mental crisis.As an energy carrier,hydrogen has been getting attention due to its abundance,high energy density,and zero carbon emission.Due to the difficulty of hydrogen storage and transport,the electro-oxidation of ammonia shows great po-tential for renewable energy since it satisfies both energy supply and environmental protection as a carbon-free fuel with high hydrogen content.However,ammonia electro-oxi-dation is a sluggish reaction and shows low durability.Un-derstanding the complicated mechanism and intermediates is conducive to developing efficient electrocatalysts with high catalytic activity and durability.This review begins with the ammonia oxidation technologies and their principles.The two typical mechanisms for ammonia electro-oxidation,Oswin-Salomon mechanism and Gerischer-Mauerer mechanism,are discussed,and attention to the poisoning species is included.Then,the electrocatalysts for ammonia reaction are classified into Pt-based catalysts and non-noble metal-based catalysts,and their performances are reviewed with various strategies.Based on the progress on the electrochemical ammonia oxi-dation catalysts,the challenges and future insight on ammonia oxidation reaction are discussed and proposed.
文献关键词:
中图分类号:
作者姓名:
Sol A Lee;Mi Gyoung Lee;Ho Won Jang
作者机构:
Department of Materials Science and Engineering,Seoul National University,Seoul 08826,Republic of Korea;Department of Electrical and Computer Engineering,University of Toronto,Toronto M5S 3G4,Ontario,Canada;Advanced Institute of Convergence Technology,Seoul National University,Suwon 16229,Republic of Korea
文献出处:
引用格式:
[1]Sol A Lee;Mi Gyoung Lee;Ho Won Jang-.Catalysts for electrochemical ammonia oxidation:Trend,challenge,and promise)[J].中国科学:材料科学(英文),2022(12):3334-3352
A类:
critial,Oswin,Salomon,Gerischer,Mauerer
B类:
Catalysts,electrochemical,ammonia,oxidation,Trend,promise,Developing,sustainable,clean,energy,nology,address,current,crisis,carrier,hydrogen,has,been,getting,attention,due,its,abundance,high,density,zero,carbon,emission,Due,difficulty,storage,transport,shows,great,tential,renewable,since,satisfies,both,supply,environmental,protection,free,fuel,content,However,sluggish,reaction,low,durability,Un,derstanding,complicated,intermediates,conducive,developing,efficient,electrocatalysts,catalytic,activity,This,begins,technologies,their,principles,two,typical,mechanisms,are,discussed,poisoning,species,included,Then,classified,into,Pt,noble,metal,performances,reviewed,various,strategies,Based,progress,challenges,future,insight,proposed
AB值:
0.492935
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