典型文献
Controlled synthesis of Pt-loaded yolk-shell TiO2@SiO2 nanoreactors as effective photocatalysts for hydrogen generation
文献摘要:
Yolk-shell and hollow structures are powerful platforms for controlled release,confined nanocatalysis,and optical and electronic applications.This contribu-tion describes a fabrication strategy for a yolk-shell nanoreactor(NR)using a post decoration approach.The widely studied yolk-shell structure of silica-coated TiO2(TiO2@SiO2)was used as a model.At first,anatase TiO2 spheres were prepared,and subsequently were given a continuous coating of carbonaceous and silica layers.Finally,the carbonaceous layer was removed to produce a yolk-shell structure TiO2@SiO2.By using an in-situ photodeposition method,Pt-encased spheres(Pt-TiO2@SiO2)were synthesized with Pt nanoparticles grown on the surface of the TiO2 core,which contained void spaces suitable for use as NRs.The NR showed enhanced hydrogen production with a rate of 24.56 mmol·g-1·h-1 in the presence of a sacrificial agent under simulated sunlight.This strategy holds the potential to be extended for the synthesis of other yolk-shell photocatalytic NRs with different metal oxides.
文献关键词:
中图分类号:
作者姓名:
Min SHI;Niannian HU;Haimei LIU;Cheng QIAN;Chang LV;Sheng WANG
作者机构:
School of Materials Science and Engineering,Zhejiang Sci-Tech University,Hangzhou 310018,China
文献出处:
引用格式:
[1]Min SHI;Niannian HU;Haimei LIU;Cheng QIAN;Chang LV;Sheng WANG-.Controlled synthesis of Pt-loaded yolk-shell TiO2@SiO2 nanoreactors as effective photocatalysts for hydrogen generation)[J].材料学前沿,2022(01):133-140
A类:
nanoreactors,nanocatalysis
B类:
Controlled,synthesis,Pt,loaded,yolk,shell,TiO2,SiO2,effective,photocatalysts,hydrogen,generation,Yolk,hollow,structures,powerful,platforms,controlled,release,confined,optical,electronic,applications,This,contribu,describes,fabrication,strategy,using,post,decoration,approach,widely,studied,silica,coated,was,used,model,At,first,anatase,spheres,were,prepared,subsequently,given,continuous,coating,carbonaceous,layers,Finally,removed,produce,By,situ,photodeposition,method,encased,synthesized,nanoparticles,grown,surface,core,which,contained,void,spaces,suitable,NRs,showed,enhanced,production,presence,sacrificial,agent,under,simulated,sunlight,holds,potential,extended,other,photocatalytic,different,metal,oxides
AB值:
0.584981
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