典型文献
Sputtering FeCu nanoalloys as active sites for alkane formation in CO2 hydrogenation
文献摘要：
Catalytic conversion of CO2 to high-value products is a crucial method to achieve targets of carbon diox-ide emissions peak and carbon neutralization.However,realizing a controllable product distribution in a single CO2 hydrogenation process is of great challenge.Herein,we prepared the CuFe nanoalloy catalyst that directly transforms CO2 to alkanes using physical sputtering method in mild condition.The charac-teristic results show that the proximity between Cu and Fe is the crucial factor to tunable products among the different catalysts.The formation of unique coordination of FeCu4 nanoalloys from high-energy sput-tering process provides close interaction between Cu and Fe,which is favorable to formation of low car-bon paraffin,however,a distant proximity and weak interaction will increase the selectivity of olefins and alcohols.This work provides a general strategy for tuning target chemicals and enriches the viewpoints in CO2 hydrogenation.
文献关键词：
中图分类号：
作者姓名：
Zhiyan Si;Cederick Cyril Amoo;Yu Han;Jian Wei;Jiafeng Yu;Qingjie Ge;Jian Sun
作者机构：
Dalian National Laboratory for Clean Energy,Dalian Institute of Chemical Physics,Chinese Academy of Sciences,Dalian 116023,Liaoning,China;University of Chinese Academy of Sciences,Beijing 100049,China
文献出处：
引用格式：
[1]Zhiyan Si;Cederick Cyril Amoo;Yu Han;Jian Wei;Jiafeng Yu;Qingjie Ge;Jian Sun-.Sputtering FeCu nanoalloys as active sites for alkane formation in CO2 hydrogenation)[J].能源化学,2022(07):162-173
A类：
nanoalloys,nanoalloy,FeCu4,sput
B类：
Sputtering,active,sites,formation,hydrogenation,Catalytic,conversion,high,value,products,crucial,method,achieve,targets,carbon,diox,emissions,peak,neutralization,However,realizing,controllable,distribution,single,process,great,challenge,Herein,prepared,CuFe,that,directly,transforms,alkanes,using,physical,sputtering,mild,condition,charac,teristic,results,show,proximity,between,tunable,among,different,catalysts,unique,coordination,from,energy,provides,close,interaction,which,favorable,low,paraffin,however,distant,weak,will,increase,selectivity,olefins,alcohols,This,work,general,strategy,tuning,chemicals,enriches,viewpoints
AB值：
0.573079
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