典型文献
Lamb-dip saturated-absorption cavity ring-down rovibrational molecular spectroscopy in the near-infrared
文献摘要:
The high-detection-sensitivity saturated-absorption cavity ring-down(SCAR)technique is extended to Lamb-dip spectroscopy of rovibrational molecular transitions in the near-infrared region.Frequency-comb-referenced sub-Doppler saturation measurements,performed on the acetylene(v1+υ3+υ4 ← υ4)R(14)e line at 6562 cm1,are analyzed by a SCAR global line profile fitting routine,based on a specially developed theoretical model.Compared to a conventional cavity ring-down evaluation,our approach yields dip profiles with a line-width freed from saturation broadening effects,reduced by 40%,and a signal-to-noise ratio increased by 90%.Ultimately,an overall(statistical and systematic)fractional uncertainty as low as 7×10-12 is achieved for the absolute line-center frequency.At the same time,our method is also able to accurately infer the linear(non-saturated)behavior of the gas absorption,providing Lamb-dip-based line strength measurements with a relative uncertainty of 0.5%.
文献关键词:
中图分类号:
作者姓名:
ROBERTO AIELLO;VALENTINA DI SARNO;MARIA GIULIA DELLI SANTI;MAURIZIO DE ROSA;IOLANDA RICCIARDI;GIOVANNI GIUSFREDI;PAOLO DE NATALE;LUIGI SANTAMARIA;PASQUALE MADDALONI
作者机构:
Consiglio Nazionale delle Ricerche-Istituto Nazionale di Ottica,Via Campi Flegrei 34,80078 Pozzuoli,Italy;Istituto Nazionale di Fisica Nucleare,Sez.di Napoli,Complesso Universitario di M.S.Angelo,Via Cintia,80126 Napoli,Italy;ppqSense S.r.I.,Via Gattinella 20,50013 Campi Bisenzio,Italy;Consiglio Nazionale delle Ricerche-Istituto Nazionale di Ottica,Largo E.Fermi 6,50125 Firenze,Italy;Agenzia Spaziale Italiana,Contrada Terlecchia,75100 Matera,Italy
文献出处:
引用格式:
[1]ROBERTO AIELLO;VALENTINA DI SARNO;MARIA GIULIA DELLI SANTI;MAURIZIO DE ROSA;IOLANDA RICCIARDI;GIOVANNI GIUSFREDI;PAOLO DE NATALE;LUIGI SANTAMARIA;PASQUALE MADDALONI-.Lamb-dip saturated-absorption cavity ring-down rovibrational molecular spectroscopy in the near-infrared)[J].光子学研究(英文),2022(08):1803-1809
A类:
rovibrational,v1+
B类:
Lamb,dip,saturated,absorption,cavity,ring,down,molecular,spectroscopy,infrared,high,detection,sensitivity,SCAR,technique,extended,transitions,region,Frequency,comb,referenced,sub,Doppler,saturation,measurements,performed,acetylene,3+,cm1,analyzed,by,global,fitting,routine,specially,developed,theoretical,model,Compared,conventional,evaluation,our,approach,yields,profiles,width,freed,from,broadening,effects,reduced,signal,noise,increased,Ultimately,overall,statistical,systematic,fractional,uncertainty,low,achieved,absolute,center,frequency,At,same,method,also,able,accurately,infer,linear,behavior,gas,providing,strength,relative
AB值:
0.566157
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