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典型文献
High-performance Ag2BiI5 Pb-free perovskite photodetector
文献摘要:
Recently, lead-free all-inorganic halide perovskites have attracted great interest because they not only have the merits of the halide perovskite family, but also are non-toxic. However, the commercialization of lead-free all-inorganic perovskites is restricted by their relatively low performances, which are usually caused by the fabrication methods and undesirable interfaces between the active layer and carrier transport layers. Herein, we demonstrate a solution-processed route for high-quality Ag2BiI5 lead-free perovskite film by adopting ideal electron transport material SnO2 and a carbon electrode. By optimizing the fabrication process and tailoring the composition of the perovskite active layer, a high-performance photodetector (PD) with an FTO/SnO2/Ag2BiI5/carbon structure PD is first fabricated, which shows good self-powered performance with a detectivity of as high as 5.3×1012 Jones and a linear dynamic range of up to 138 dB, which are better than those of the reported Pb-free perovskite PDs and comparable to high-performance Pb-based perovskite PDs. In addition, our unpackaged PDs show good light, thermal, and storage stability in air. Our results provide a special route for the development of lead-free perovskite devices in an environmentally friendly field.
文献关键词:
作者姓名:
Zihao Shuang;Hai Zhou;Dingjun Wu;Xuhui Zhang;Boao Xiao;Jinxia Duan;Hao Wang
作者机构:
International School of Microelectronics, Dongguan University of Technology, Dongguan 523808, China;Hubei Yangtze Memory Laboratories, Wuhan 430205, China;School of Microelectronics, Hubei University, Wuhan 430062, China;e-mail: hizhou@dgut.edu.cn;e-mail: wangh@hubu.edu.cn
引用格式:
[1]Zihao Shuang;Hai Zhou;Dingjun Wu;Xuhui Zhang;Boao Xiao;Jinxia Duan;Hao Wang-.High-performance Ag2BiI5 Pb-free perovskite photodetector)[J].光子学研究(英文),2022(08):1886
A类:
Ag2BiI5,unpackaged
B类:
High,Pb,free,photodetector,Recently,lead,inorganic,halide,perovskites,have,attracted,great,interest,because,they,not,only,merits,family,but,also,are,toxic,However,commercialization,is,restricted,by,their,relatively,low,performances,which,usually,caused,fabrication,methods,undesirable,interfaces,between,active,carrier,transport,layers,Herein,demonstrate,solution,processed,route,high,quality,film,adopting,ideal,electron,material,SnO2,carbon,electrode,By,optimizing,tailoring,composition,FTO,structure,first,fabricated,shows,good,self,powered,detectivity,Jones,linear,dynamic,range,up,dB,better,than,those,reported,PDs,comparable,In,addition,our,light,thermal,storage,stability,air,Our,results,provide,special,development,devices,environmentally,friendly,field
AB值:
0.558841
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