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典型文献
Coupling of piezocatalysis and photocatalysis for efficient degradation of methylene blue by Bi0.9Gd0.07La0.03FeO3 nanotubes
文献摘要:
Photocatalytic degradation of organic pollutants is of great significance for wastewater remediation but is still hindered by the poor catalytic efficiency of the catalysts.Herein,we report a strategy to simultaneously introduce piezocatalysis and to enhance the intrinsic photocatalysis in a single catalyst,which improved the performance for catalytic degradation of methylene blue(MB)significantly.Specifically,piezoelectric BiFeO3(BFO)nanotube doped with different contents of Gd and La(Bi0.9(Gd,La1-x)0.1FeO3)were produced by electrospinning.The doping led to a higher concentration of surface oxygen vacancy(OV)in Bi0.9Gd0.07La0.03FeO3,which effectively increased the piezoelectric field due to the deformation of BFO,and suppressed the recombination of photon-generated electron-hole pairs.The Bi0.9Gd0.07La0.03FeO3 nanotube showed excellent catalytic performance under simultaneous light irradiation and ultrasonic excitation,giving an extraordinary 95%degradation of MB within 90 min.These findings suggest that the piezoelectric effect combined with defect engineering can enhance the catalytic performance of Bi0.9Gd0.07La0.03FeO3 nanotube.This could potentially be extended to other catalytic systems for high-performance pollutant treatment.
文献关键词:
作者姓名:
Angom Devadatta MANI;Jie LI;Ziquan WANG;Jiale ZHOU;Huaicheng XIANG;Jinlai ZHAO;Libo DENG;Haitao YANG;Lei YAO
作者机构:
Shenzhen Key Laboratory of Special Functional Materials,Shenzhen Engineering Laboratory for Advanced Technology of Ceramics,Guangdong Research Center for Interfacial Engineering of Functional Materials,College of Materials Science and Engineering,Shenzhen University,Shenzhen 518071,China;Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province,College of Optoelectronic Engineering,Shenzhen University,Shenzhen 518060,China;College of Chemistry and Environmental Engineering,Shenzhen University,Shenzhen 518071,China
引用格式:
[1]Angom Devadatta MANI;Jie LI;Ziquan WANG;Jiale ZHOU;Huaicheng XIANG;Jinlai ZHAO;Libo DENG;Haitao YANG;Lei YAO-.Coupling of piezocatalysis and photocatalysis for efficient degradation of methylene blue by Bi0.9Gd0.07La0.03FeO3 nanotubes)[J].先进陶瓷(英文版),2022(07):1069-1081
A类:
07La0,03FeO3,1FeO3
B类:
Coupling,piezocatalysis,photocatalysis,efficient,degradation,methylene,blue,by,Bi0,9Gd0,nanotubes,Photocatalytic,organic,pollutants,great,significance,wastewater,remediation,but,still,hindered,poor,efficiency,catalysts,Herein,report,strategy,simultaneously,introduce,enhance,intrinsic,single,which,improved,performance,MB,significantly,Specifically,piezoelectric,BiFeO3,BFO,doped,different,contents,La1,were,produced,electrospinning,doping,led,higher,concentration,surface,oxygen,vacancy,OV,effectively,increased,field,due,deformation,suppressed,recombination,photon,generated,electron,hole,pairs,showed,excellent,under,light,irradiation,ultrasonic,excitation,giving,extraordinary,within,These,findings,suggest,that,combined,defect,engineering,This,could,potentially,extended,other,systems,treatment
AB值:
0.516649
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