典型文献
Highly dispersed CeO2-x nanoparticles with rich oxygen vacancies enhance photocatalytic performance of g-C3N4 toward methyl orange degradation under visible light irradiation
文献摘要:
CeO2/g-C3N4 photocatalysts have attracted tremendous attention in the photocatalytic degradation of organic pollutants.The design and construction of highly active CeO2/g-C3N4 photocatalysts without harsh conditions are still challenging.Herein,highly dispersed CeO2-x nanoparticles with rich oxygen vacancies were successfully precipitated on the surface of g-C3N4 under mild conditions.The fabricated CeO2-x/g-C3N4 exhibits remarkable activity and stability for photocatalytic degradation of MO pollutant.The optimal rate constant of MO degradation over CeO2-x/g-C3N4 is about 0.031 min-1,which is three times higher than that of g-C3N4.A negligible activity decrease is observed after three cycling runs.The enhanced catalytic performance can be ascribed to the excellent dispersion of CeO2-x with rich oxygen vacancies that benefit O2 adsorption and visible light absorption.In addition,the proper band alignment between CeO2-x and g-C3N4 is conducive to the highly efficient separation of photogenerated electron-hole pairs.
文献关键词:
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作者姓名:
Xuejun Xu;Tianhua Huang;Yisheng Xu;Huawen Hu;Shuang Liao;Xiaohong Hu;Dongchu Chen;Min Zhang
作者机构:
School of Materials Science and Hydrogen Energy,Foshan University,Foshan 528000,China;Guangdong Key Laboratory for Hydrogen Energy Technologies,Foshan 528000,China
文献出处:
引用格式:
[1]Xuejun Xu;Tianhua Huang;Yisheng Xu;Huawen Hu;Shuang Liao;Xiaohong Hu;Dongchu Chen;Min Zhang-.Highly dispersed CeO2-x nanoparticles with rich oxygen vacancies enhance photocatalytic performance of g-C3N4 toward methyl orange degradation under visible light irradiation)[J].稀土学报(英文版),2022(08):1255-1263
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Highly,dispersed,CeO2,nanoparticles,rich,oxygen,vacancies,photocatalytic,performance,C3N4,toward,methyl,orange,degradation,under,visible,light,irradiation,photocatalysts,have,attracted,tremendous,attention,organic,pollutants,design,construction,highly,active,without,harsh,conditions,are,still,challenging,Herein,were,successfully,precipitated,surface,mild,fabricated,exhibits,remarkable,activity,stability,MO,optimal,constant,over,about,which,three,times,higher,than,that,negligible,decrease,observed,after,cycling,runs,enhanced,ascribed,excellent,dispersion,benefit,adsorption,absorption,In,addition,proper,band,alignment,between,conducive,efficient,separation,photogenerated,electron,hole,pairs
AB值:
0.571594
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