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典型文献
Ni3N Modified MOF Heterostructure with Tailored Electronic Struc-ture for Efficient Overall Water Splitting
文献摘要:
Exploring bifunctional electrocatalysts with high-efficiency and stability toward overall water splitting is desirable for sustainable energy technologies,yet challenging.Herein,we report the construction of Ni3N on the surface of Ni-MOF-74 through an in-situ nitriding process.The obtained Ni-MOF-74/Ni3N exhibits remarkable HER activity with an overpotential of 73 mV to deliver 10 mA cm-2.Theoretical calculations and experimental study demonstrate the electron transport between Ni3N and Ni-MOF-74,leading to the im-proved H2O adsorption,optimized hydrogen adsorption,and increased Had diffusion,which contributes to the enhanced HER performance.Besides,the obtained Ni-MOF-74/Ni3N also possesses outstanding activity toward OER and overall water splitting.
文献关键词:
作者姓名:
Hongnan Jia;Na Yao;Juan Zhu;Yujia Liu;Yunhao Lao;Hengjiang Cong;Wei Luo
作者机构:
College of Chemistry and Molecular Sciences,Wuhan University,Wuhan 430072,China;Suzhou Institute of Wuhan University,Suzhou,Jiangsu 215123,China
文献出处:
引用格式:
[1]Hongnan Jia;Na Yao;Juan Zhu;Yujia Liu;Yunhao Lao;Hengjiang Cong;Wei Luo-.Ni3N Modified MOF Heterostructure with Tailored Electronic Struc-ture for Efficient Overall Water Splitting)[J].结构化学,2022(08):31-36
A类:
Struc
B类:
Ni3N,Modified,MOF,Heterostructure,Tailored,Electronic,Efficient,Overall,Water,Splitting,Exploring,bifunctional,electrocatalysts,high,efficiency,stability,toward,overall,water,splitting,is,desirable,sustainable,energy,technologies,yet,challenging,Herein,report,construction,surface,through,situ,nitriding,process,obtained,exhibits,remarkable,HER,activity,overpotential,mV,deliver,mA,Theoretical,calculations,experimental,study,demonstrate,electron,transport,between,leading,proved,H2O,adsorption,optimized,hydrogen,increased,Had,diffusion,which,contributes,enhanced,performance,Besides,also,possesses,outstanding,OER
AB值:
0.646896
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