典型文献
Efficient photoelectrodes based on two-dimensional transition metal dichalcogenides heterostructures:from design to construction
文献摘要:
Hydrogen production by photoelectrochemical(PEC)water splitting converts the inexhaustible supply of solar radiation to storable H2 as clean energy and thus has received widespread attention.The efficiency of PEC water splitting is largely determined by the properties of the photoelectrodes.Two-dimensional(2D)layered transition metal dichalcogenides(TMDs)are promising candidates for photoelectrodes due to their atomic layer thickness,tunable bandgap,large specific surface area,and high carrier mobility.Moreover,the construction of 2D TMDs heterostructures provides freedom in material design,which facilitates the further improvement of PEC water splitting.This review begins by describing the mechanism of PEC water splitting and the advantages of 2D TMD-based heterostructures for photoelectrodes.Then,the design considerations of the heterostructures for enhanced PEC efficiency are comprehensively reviewed with a focus on material selection,band engineering,surface modifica-tion,and long-term durability.Finally,current challenges and future perspectives for the development of photoelec-trodes based on 2D TMDs heterostructures are addressed.
文献关键词:
中图分类号:
作者姓名:
Xiang-Chao Lu;Yi-Zhen Lu;Cong Wang;Yang Cao
作者机构:
State Key Laboratory of Physical Chemistry of Solid Surfaces,Collaborative Innovation Center of Chemistry for Energy Materials(iChEM),College of Chemistry and Chemical Engineering,Xiamen University,Xiamen 361005,China;Pen-Tung Sah Institute of Micro-Nano Science and Technology,Xiamen University,Xiamen 361005,China
文献出处:
引用格式:
[1]Xiang-Chao Lu;Yi-Zhen Lu;Cong Wang;Yang Cao-.Efficient photoelectrodes based on two-dimensional transition metal dichalcogenides heterostructures:from design to construction)[J].稀有金属(英文版),2022(04):1142-1159
A类:
inexhaustible
B类:
Efficient,photoelectrodes,two,dimensional,transition,metal,dichalcogenides,heterostructures,from,design,construction,Hydrogen,production,by,photoelectrochemical,PEC,water,splitting,converts,supply,solar,radiation,storable,H2,clean,energy,thus,has,received,widespread,attention,efficiency,largely,determined,properties,Two,2D,layered,TMDs,promising,candidates,due,their,atomic,thickness,tunable,bandgap,specific,surface,area,high,carrier,mobility,Moreover,provides,freedom,material,which,facilitates,further,improvement,This,begins,describing,mechanism,advantages,Then,considerations,enhanced,comprehensively,reviewed,focus,selection,engineering,modifica,long,durability,Finally,current,challenges,future,perspectives,development,addressed
AB值:
0.543101
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