典型文献
Modulate the superficial structure of La2Ce2O7 catalyst with anchoring CuOx species for the selective catalytic oxidation of NH3
文献摘要:
Air contamination caused by the ammonia slip phenomenon has gradually captured the researcher's ex-tensive attention.An effective strategy for controlling fugitive NH3 is critical to improving the air quality and living environment.In the present work,CuOx/La2Ce2O7 composite as a potential candidate catalyst is synthesized through the electrostatic adsorption method for the selective catalytic oxidation(SCO)of NH3 to N2.The 5%CuOx/La2Ce2O7 exhibits the best catalytic activity(T90=243℃)and ammonia con-version efficiency.The improvement of performance is mainly attributed to the superficial connection of[Ce-O-Cu],which enhances the capturing ability of ammonia molecule and accelerates the dissociating efficiency of N-H bonding for N2 evolution,simultaneously.This work provides a facile method to syn-thesis pyrochlore-like composite catalyst of NH3-SCO for solving the problem of ammonia slip pollution in the future.
文献关键词:
中图分类号:
作者姓名:
Xiangchen Kong;Zhenguo Li;Yuankai Shao;Xiaoning Ren;Kaixiang Li;Hanming Wu;Congjie Lv;Cheng Lv;Shengli Zhu
作者机构:
National Engineering Laboratory for Mobile Source Emission Control Technology,China Automotive Technology&Research Center Co.,Ltd.,Tianjin 300300,China;School of Materials Science and Engineering,Tianjin University,Tianjin 300350,China;School of Materials Science and Engineering,Lanzhou Jiaotong University,Lanzhou 730070,China
文献出处:
引用格式:
[1]Xiangchen Kong;Zhenguo Li;Yuankai Shao;Xiaoning Ren;Kaixiang Li;Hanming Wu;Congjie Lv;Cheng Lv;Shengli Zhu-.Modulate the superficial structure of La2Ce2O7 catalyst with anchoring CuOx species for the selective catalytic oxidation of NH3)[J].材料科学技术(英文版),2022(16):1-8
A类:
La2Ce2O7,dissociating
B类:
Modulate,superficial,structure,catalyst,anchoring,CuOx,species,selective,catalytic,oxidation,NH3,Air,contamination,caused,by,ammonia,slip,phenomenon,has,gradually,captured,researcher,tensive,attention,An,effective,strategy,controlling,fugitive,critical,improving,air,quality,living,environment,In,present,work,composite,potential,candidate,synthesized,through,electrostatic,adsorption,method,SCO,N2,exhibits,best,activity,T90,version,efficiency,improvement,performance,mainly,attributed,connection,which,enhances,capturing,ability,molecule,accelerates,bonding,evolution,simultaneously,This,provides,facile,thesis,pyrochlore,like,solving,problem,pollution,future
AB值:
0.588009
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