典型文献
Effect of Particle Shape on Catalyst Deactivation during 2-Butene and Isobutane Alkylation of Liquid Phase in Fixed-Bed Reactor Using Particle-Resolved CFD Simulation
文献摘要：
How catalyst shape affects its deactivation is a crucial issue for quickly decaying catalysts such as zeolite in 2-butene and isobutane alkylation.In this work,steady simulations are used to determine the temperature and species distribution in fixed beds filled with particles of four shapes.Subsequently,unsteady simulations are used to study the deactivation behavior of the catalysts based on the steady simulation results.We describe the deactivation rate and type of catalyst deactivation by defining a local internal diffusivity,which is affected by catalytic activity.The results reveal that the internal diffusion distance of the catalyst determines the deactivation rate,whereas the local internal diffusivity determines its deactivation type.
文献关键词：
中图分类号：
作者姓名：
Zhang Sizhen;Zhu Zhenxing;Xin Feng;Chu Menghan
作者机构：
School of Chemical Engineering and Technology,Tianjin University,Tianjin 300350,China;SINOPEC Research Institute of Petroleum Processing Co.,Ltd.,Beijing 100083,China
文献出处：
引用格式：
[1]Zhang Sizhen;Zhu Zhenxing;Xin Feng;Chu Menghan-.Effect of Particle Shape on Catalyst Deactivation during 2-Butene and Isobutane Alkylation of Liquid Phase in Fixed-Bed Reactor Using Particle-Resolved CFD Simulation)[J].中国炼油与石油化工（英文版）,2022(04):139-150
A类：
Deactivation,Isobutane
B类：
Effect,Particle,Shape,Catalyst,during,Butene,Alkylation,Liquid,Phase,Fixed,Bed,Reactor,Using,Resolved,CFD,Simulation,How,affects,its,deactivation,crucial,issue,quickly,decaying,catalysts,such,zeolite,butene,isobutane,alkylation,In,this,work,simulations,are,used,temperature,species,distribution,fixed,beds,filled,particles,four,shapes,Subsequently,unsteady,study,behavior,results,We,describe,rate,type,by,defining,local,internal,diffusivity,which,affected,catalytic,activity,reveal,that,diffusion,distance,determines,whereas
AB值：
0.597232
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