Lumbini is a world heritage site located in the southern plains region of Nepal,and is regarded as a poten-tial site for evaluating transboundary air pollution due to its proximity to the border with India.In this study,82 aerosol samples were collected between April 2013 and July 2014 to investigate the levels of particulate-bound mercury (PBM) and the corresponding seasonality,sources,and influencing factors.The PBM concentration in total suspended particulate (TSP) matter ranged from 6.8 pg m-3 to 351.7 pg m-3 (mean of 99.7 ± 92.6 pg m-3),which exceeded the ranges reported for remote and rural sites worldwide.The Hg content (PBM/TSP) ranged from 68.2 ng g-1 to 1744.8 ng g-1 (mean of 446.9 ±312.7 ng g-1),indicating anthropogenic enrichment.The PBM levels were higher in the dry season (i.e.,winter and the pre-monsoon period) than in the wet season (i.e.,the monsoon period).In addition,the δ202Hg signature indicated that waste/coal burning and traffic were the major sources of Hg in Lumbini during the pre-monsoon period.Meanwhile,precipitation occurring during photochemical pro-cesses in the atmosphere may have been responsible for the observed Δ199Hg values in the aerosol sam-ples obtained during the monsoon period.The PBM concentration was influenced mostly by the resuspension of polluted dust during dry periods and crop residue burning during the post-monsoon per-iod.The estimated PBM deposition flux at Lumbini was 15.7 μg m-2 yr-1.This study provides a reference dataset of atmospheric PBM over a year,which can be useful for understanding the geochemical cycling of Hg in this region of limited data.

Junming Guo;Lekhendra Tripathee;Shichang Kang;Qianggong Zhang;Jie Huang;Chhatra Mani Sharma;Pengfei Chen;Rukumesh Paudyal;Dipesh Rupakheti

State Key Laboratory of Cryospheric Science,Northwest Institute of Eco-Environment and Resources,Chinese Academy of Sciences,Lanzhou 730000,China;Himalayan Environment Research Institute (HERI),Kathmandu,Nepal;Center for Excellence in Tibetan Plateau Earth Sciences,Chinese Academy of Sciences,Beijing 100085,China;University of Chinese Academy of Sciences,Beijing 100039,China;Key Laboratory of Tibetan Environment Changes and Land Surface Processes,Institute of Tibetan Plateau Research,Chinese Academy of Sciences,Beijing 100101,China;Central Department of Environmental Science,Tribhuvan University,Kathmandu,Nepal

地学前缘（英文版）

[1]Junming Guo;Lekhendra Tripathee;Shichang Kang;Qianggong Zhang;Jie Huang;Chhatra Mani Sharma;Pengfei Chen;Rukumesh Paudyal;Dipesh Rupakheti-.Atmospheric particle-bound mercury in the northern Indo-Gangetic Plain region:Insights into sources from mercury isotope analysis and influencing factors)[J].地学前缘（英文版）,2022(01):85-95

Lumbini,iod

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