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典型文献
Isotype Heterojunction-Boosted CO2 Photoreduction to CO
文献摘要:
Photocatalytic conversion of CO2 to high-value products plays a crucial role in the global pursuit of carbon-neutral economy.Junction photocatalysts,such as the isotype heterojunctions,offer an ideal paradigm to navigate the photocatalytic CO2 reduction reaction(CRR).Herein,we elucidate the behaviors of isotype heterojunctions toward photocatalytic CRR over a representative photocatalyst,g-C3N4.Impressively,the isotype heterojunctions possess a significantly higher efficiency for the spatial separation and transfer of photogenerated car-riers than the single components.Along with the intrinsically outstand-ing stability,the isotype heterojunctions exhibit an exceptional and stable activity toward the CO2 photoreduction to CO.More importantly,by combining quantitative in situ technique with the first-principles modeling,we elucidate that the enhanced photoinduced charge dynamics promotes the production of key intermediates and thus the whole reaction kinetics.
文献关键词:
作者姓名:
Chaogang Ban;Youyu Duan;Yang Wang;Jiangping Ma;Kaiwen Wang;Jiazhi Meng;Xue Liu;Cong Wang;Xiaodong Han;Guozhong Cao;Liyong Gan;Xiaoyuan Zhou
作者机构:
College of Physics and Center of Quantum Materials and Devices,Chongqing University,Chongqing 401331,People's Republic of China;Beijing Key Laboratory of Microstructure and Property of Advanced Materials,Beijing University of Technology,Beijing 100024,People's Republic of China;Department of Materials Science and Engineering,University of Washington,Seattle,WA 98195,USA;State Key Laboratory of Coal Mine Disaster Dynamics and Control,Chongqing University,Chongqing 401331,People's Republic of China;Analytical and Testing Center,Chongqing University,Chongqing 401331,People's Republic of China
引用格式:
[1]Chaogang Ban;Youyu Duan;Yang Wang;Jiangping Ma;Kaiwen Wang;Jiazhi Meng;Xue Liu;Cong Wang;Xiaodong Han;Guozhong Cao;Liyong Gan;Xiaoyuan Zhou-.Isotype Heterojunction-Boosted CO2 Photoreduction to CO)[J].纳微快报(英文),2022(05):97-109
A类:
Isotype
B类:
Heterojunction,Boosted,Photoreduction,Photocatalytic,conversion,value,products,plays,crucial,role,global,pursuit,carbon,neutral,economy,Junction,photocatalysts,such,as,isotype,heterojunctions,offer,ideal,paradigm,navigate,photocatalytic,reaction,CRR,Herein,we,elucidate,behaviors,toward,over,representative,C3N4,Impressively,possess,significantly,higher,efficiency,spatial,separation,transfer,photogenerated,riers,than,single,components,Along,intrinsically,outstand,stability,exhibit,exceptional,stable,activity,photoreduction,More,importantly,by,combining,quantitative,situ,technique,first,principles,modeling,that,enhanced,photoinduced,charge,dynamics,promotes,production,key,intermediates,thus,whole,kinetics
AB值:
0.67569
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