典型文献
Role of different types of water in bentonite clay on hydrate formation and decomposition
文献摘要:
The equilibrium and kinetic of hydrate in sediments can be affected by the presence of external compo-nents like bentonite with a relatively large surface area.To investigate the hydrate formation and decom-position behaviors in bentonite clay,the experiments of methane hydrate formation and decomposition using the multi-step decomposition method in bentonite with different water contents of 20%,40%and 60%(mass)were carried out.The contents of bound,capillary and gravity water in bentonite clay and their roles during hydrate formation and decomposition were analyzed.In bentonite with water content of 20%(mass),the hydrate formation rate keeps fast during the whole formation process,and the final gas consumption under different initial formation pressures is similar.In bentonite with the water contents of 40%and 60%(mass),the hydrate formation rate declines significantly at the later stage of the hydrate formation.The final gas consumption of bentonite with the water contents of 40%and 60%(mass)is sig-nificantly higher than that with the water content of 20%(mass).During the decomposition process,the stable pressure increases with the decrease of the water content.Hydrate mainly forms in free water in bentonite clay.In bentonite clay with the water contents of 20%and 40%(mass),the hydrate forms in capillary water.In bentonite clay with the water content of 60%(mass),the hydrate forms both in cap-illary water and gravity water.The bound water of dry bentonite clay is about 3.93%(mass)and the con-tent of capillary water ranges from 42.37%to 48.21%(mass)of the dry bentonite clay.
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作者姓名:
Yu Zhang;Lei Zhang;Chang Chen;Hao-Peng Zeng;Xiao-Sen Li;Bo Yang
作者机构:
Key Laboratory of Gas Hydrate,Guangzhou Institute of Energy Conversion,Chinese Academy of Sciences,Guangzhou,Guangdong 510640,China;Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development,Guangzhou,Guangdong 510640,China;University of Chinese Academy of Sciences,Beijing 10083,China;Guangzhou Special Pressure Equipment Inspection and Research Institute,Guangzhou 510663,China
文献出处:
引用格式:
[1]Yu Zhang;Lei Zhang;Chang Chen;Hao-Peng Zeng;Xiao-Sen Li;Bo Yang-.Role of different types of water in bentonite clay on hydrate formation and decomposition)[J].中国化学工程学报(英文版),2022(10):310-316
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0.3209
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