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典型文献
Design and experiment of high-productivity two-stage vacuum pressure swing adsorption process for carbon capturing from dry flue gas
文献摘要:
A two-stage vacuum pressure swing adsorption(VPSA)process that coupled kinetically controlled and equilibrium controlled separation process with reflux has been investigated for capturing carbon dioxide from dry flue gas(85%N2/15%CO2).In the first enriching stage,carbon molecular sieve(CMS),which shows kinetic selectivity for CO2/N2,is adopted as the adsorbent to remove most N2 in feed gas,thereby upgrading CO2 and significantly reducing the amount for further refinement.The second stage loads zeo-lite 13X as adsorbent to purify the CO2-rich flow from the first stage for meeting the requirements of National Energy Technology Laboratory.Series of experiments have been conducted for adsorption iso-therms measuring and lab-scale experimental validation as well as analysis.The effect of feed composi-tion on the separation performance of the PSA system was studied experimentally and theoretically here.The optimal results achieved 95.1%purity and 92.9%recovery with a high CO2 productivity(1.89 mol CO2·h-1·kg-1)and an appropriate energy consumption of 1.07 MJ·(kg CO2)-1.Further analysis has been carried out by simulation for explicating the temperature,pressure,and concentration distribution at cyclic steady state.
文献关键词:
作者姓名:
Xiuxin Yu;Bing Liu;Yuanhui Shen;Donghui Zhang
作者机构:
The Research Center of Chemical Engineering,School of Chemical Engineering and Technology,Tianjin University,Tianjin 300072,China
引用格式:
[1]Xiuxin Yu;Bing Liu;Yuanhui Shen;Donghui Zhang-.Design and experiment of high-productivity two-stage vacuum pressure swing adsorption process for carbon capturing from dry flue gas)[J].中国化学工程学报(英文版),2022(03):378-391
A类:
zeo,therms,explicating
B类:
Design,high,productivity,two,stage,vacuum,pressure,swing,adsorption,process,carbon,capturing,from,dry,flue,gas,VPSA,that,coupled,kinetically,controlled,equilibrium,separation,reflux,has,been,investigated,dioxide,N2,In,first,enriching,molecular,sieve,CMS,which,shows,selectivity,adopted,adsorbent,remove,most,feed,thereby,upgrading,significantly,reducing,amount,further,refinement,second,loads,lite,13X,purify,flow,meeting,requirements,National,Energy,Technology,Laboratory,Series,experiments,have,conducted,iso,measuring,lab,scale,validation,well,analysis,effect,composi,performance,system,was,studied,experimentally,theoretically,optimal,results,achieved,purity,recovery,appropriate,energy,consumption,MJ,Further,carried,out,simulation,temperature,concentration,distribution,cyclic,steady,state
AB值:
0.584006
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