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典型文献
Ultrafast Coulomb explosion imaging of molecules and molecular clusters
文献摘要:
Taking an image of their structure and a movie of their dynamics of small quantum systems have always been a dream of physicists and chemists.Laser-induced Coulomb explosion imaging(CEI)provides a great opportunity to make this dream a reality for small molecules or their aggregation—clusters.The method is unique for identifying the atomic locations with ?ngstrom spatial resolution and capturing the structural evolution with a femtosecond time scale,in particular for imaging transient state products.This review summarizes the determination of three-dimensional equilibrium geometry of molecules and molecular cluster system through the reconstruction from the fragments momenta,and also shows that the dissociation dynamics on the complex potential energy surface can be tracked in real-time with the ultrafast CEI(UCEI).Furthermore,the detailed measurement and analysis procedures of the CEI,theoretical methods,exemplary results,and future perspectives of the technique are described.
文献关键词:
作者姓名:
Xiaokai Li;Xitao Yu;Pan Ma;Xinning Zhao;Chuncheng Wang;Sizuo Luo;Dajun Ding
作者机构:
Institute of Atomic and Molecular Physics,Jilin University,Changchun 130012,China
引用格式:
[1]Xiaokai Li;Xitao Yu;Pan Ma;Xinning Zhao;Chuncheng Wang;Sizuo Luo;Dajun Ding-.Ultrafast Coulomb explosion imaging of molecules and molecular clusters)[J].中国物理B(英文版),2022(10):9-23
A类:
ngstrom,UCEI
B类:
Ultrafast,Coulomb,explosion,imaging,molecules,molecular,clusters,Taking,image,their,structure,movie,dynamics,small,quantum,systems,have,always,been,dream,physicists,chemists,Laser,induced,provides,great,opportunity,make,this,reality,aggregation,unique,identifying,atomic,locations,spatial,resolution,capturing,structural,evolution,femtosecond,scale,particular,transient,state,products,This,review,summarizes,determination,three,dimensional,equilibrium,geometry,through,reconstruction,from,fragments,momenta,also,shows,that,dissociation,complex,potential,energy,surface,can,tracked,ultrafast,Furthermore,detailed,measurement,analysis,procedures,theoretical,methods,exemplary,results,future,perspectives,technique,are,described
AB值:
0.651744
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