典型文献
Promotion effect of sulfur impurity in alumina support on propane dehydrogenation
文献摘要：
Alumina materials are widely applied either as a catalyst or support in various industrial catalytic pro-cesses.Impurities in alumina that are unfriendly to catalytic performance are inevitably present during the production processes.Facing this problem,we here report that the use of sulfur-containing alumina as the support can generate active alumina-supported platinum catalyst,which exhibits superior propy-lene selectivity and anti-coking ability during propane dehydrogenation.It demonstrated that the sulfur impurity in alumina is not entirely detrimental.During the reduction process,the formation of gas-phase sulfur species increased the electrons and poisoned unsaturated sites of platinum particles.The sulfur impurity in alumina can be removed through a hydrogen reduction process,and the degree of desulfur-ization is correlated with the operating temperature.This study demonstrated that the rational use of impurity will contribute to the design of a catalyst with high reactivity for potential applications.
文献关键词：
中图分类号：
作者姓名：
Xin-Qian Gao;Wen-Cui Li;Bin Qiu;Jian Sheng;Fan Wu;An-Hui Lu
作者机构：
State Key Laboratory of Fine Chemicals,School of Chemical Engineering,Dalian University of Technology,Dalian 116024,Liaoning,China
文献出处：
引用格式：
[1]Xin-Qian Gao;Wen-Cui Li;Bin Qiu;Jian Sheng;Fan Wu;An-Hui Lu-.Promotion effect of sulfur impurity in alumina support on propane dehydrogenation)[J].能源化学,2022(07):332-339
A类：
Impurities,propy,desulfur
B类：
Promotion,effect,impurity,alumina,propane,dehydrogenation,Alumina,materials,are,widely,applied,either,catalyst,various,industrial,catalytic,that,unfriendly,performance,inevitably,present,during,production,processes,Facing,this,problem,we,here,report,use,containing,can,generate,active,supported,platinum,which,exhibits,superior,lene,selectivity,anti,coking,ability,It,demonstrated,not,entirely,detrimental,During,reduction,formation,gas,phase,species,increased,electrons,poisoned,unsaturated,sites,particles,be,removed,through,degree,ization,correlated,operating,temperature,This,study,rational,will,contribute,design,high,reactivity,potential,applications
AB值：
0.556125
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