典型文献
Is atmospheric oxidation capacity better in indicating tropospheric O3 formation?
文献摘要:
Tropospheric ozone(O3)concentration is increasing in China along with dramatic changes in precursor emissions and meteorological conditions,adversely affecting human health and ecosystems.O3 is formed from the complex nonlinear photochemical reactions from nitrogen oxides(NOx=NO+NO2)and volatile organic compounds(VOCs).Although the mechanism of O3 formation is rather clear,describing and analyzing its changes and formation potential at fine spatial and temporal resolution is still a challenge today.In this study,we briefly summarized and evaluated different approaches that indicate O3 formation regimes.We identify that atmospheric oxidation capacity(AOC)is a better indicator of photochemical reactions leading to the formation of O3 and other secondary pollutants.Results show that AOC has a prominent positive relationship to O3 in the major city clusters in China,with a goodness of fit(R2)up to 0.6.This outcome provides a novel perspective in characterizing O3 formation and has significant implications for formulating control strategies of secondary pollutants.
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作者姓名:
Peng Wang;Shengqiang Zhu;Mihalis Vrekoussis;Guy P.Brasseur;Shuxiao Wang;Hongliang Zhang
作者机构:
Department of Atmospheric and Oceanic Sciences,Fudan University,Shanghai 200438,China;IRDR ICoE on Risk Interconnectivity and Governance on Weather/Climate Extremes Impact and Public Health,Fudan University,Shanghai 200438,China;Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,Department of Environmental Science&Engineering,Fudan University,Shanghai 200438,China;Institute of Environmental Physics,University of Bremen,Bremen D-28359,Germany;Climate and Atmosphere Research Center(CARE-C),the Cyprus Institute,Nicosia 27456,Cyprus;Max Planck Institute for Meteorology,Hamburg 20146,Germany;National Center for Atmospheric Research,Boulder,CO 80307,USA;State Key Joint Laboratory of Environmental Simulation and Pollution Control,School of Environment,Tsinghua University,Beijing 100084,China;State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex,Beijing 100084,China;Institute of Eco-Chongming(IEC),Shanghai 202162,China
文献出处:
引用格式:
[1]Peng Wang;Shengqiang Zhu;Mihalis Vrekoussis;Guy P.Brasseur;Shuxiao Wang;Hongliang Zhang-.Is atmospheric oxidation capacity better in indicating tropospheric O3 formation?)[J].环境科学与工程前沿,2022(05):127-133
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AB值:
0.692577
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