首站-论文投稿智能助手
典型文献
Selective introduction of surface defects in anatase TiO2 nanosheets for highly efficient photocatalytic hydrogen generation
文献摘要:
Defect engineering greatly enhances the cat-alytic activity of transition metal semiconductor photocat-alysts.Recently,localized surface defects engineering has been intensively researched,but it still remains challenges on how to tilt the balance to the controllable construction of surface defects rather than bulk ones.Here,we report a facile room-temperature solution processing strategy on(001)facet exposed anatase TiO2 nanosheets(ATO),in which localized defects are generated on the surface selectivity with high concentration.To achieve the aspect,lithium-ethylenediamine(Li-EDA)treatment is carried out on(001)facet exposed ATO under a mild condition.The optimized sample exhibits outstanding photocatalytic H2 production rates of 9.28 mmol·g-1·h-1 with loading 0.5 wt%Pt as co-catalyst(AM 1.5),which is nearly 7.5 times higher than that of the pristine ATO.This defect engi-neering strategy of ATO photocatalyst will spark the ideas for the defects engineering and semiconductor photocata-lyst,which is with important application prospect in solar energy conversion,including hydrogen generation and carbon dioxide reduction.
文献关键词:
作者姓名:
Jiang-Yuan Qiu;Hua-Zhang Feng;Zhao-Hui Chen;Shu-Hong Ruan;Yan-Ping Chen;Ting-Ting Xu;Jing-Yun Su;En-Na Ha;Lu-Yang Wang
作者机构:
College of New Materials and New Energies,Shenzhen Technology University,Shenzhen 518118,China;College of Health Science and Environmental Engineering,Shenzhen Technology University,Shenzhen 518118,China
引用格式:
[1]Jiang-Yuan Qiu;Hua-Zhang Feng;Zhao-Hui Chen;Shu-Hong Ruan;Yan-Ping Chen;Ting-Ting Xu;Jing-Yun Su;En-Na Ha;Lu-Yang Wang-.Selective introduction of surface defects in anatase TiO2 nanosheets for highly efficient photocatalytic hydrogen generation)[J].稀有金属(英文版),2022(06):2074-2083
A类:
B类:
Selective,introduction,surface,defects,anatase,TiO2,nanosheets,highly,efficient,photocatalytic,hydrogen,generation,Defect,engineering,greatly,enhances,activity,transition,metal,semiconductor,alysts,Recently,localized,has,been,intensively,researched,but,still,remains,challenges,how,tilt,balance,controllable,construction,rather,than,bulk,ones,Here,we,report,facile,room,temperature,solution,processing,strategy,facet,exposed,ATO,which,are,generated,selectivity,concentration,To,achieve,aspect,lithium,ethylenediamine,Li,EDA,treatment,carried,under,mild,condition,optimized,sample,exhibits,outstanding,H2,production,rates,loading,wt,Pt,AM,nearly,times,higher,that,pristine,This,photocatalyst,will,spark,ideas,important,application,prospect,solar,energy,conversion,including,carbon,dioxide,reduction
AB值:
0.619036
相似文献
Interface engineering of snow-like Ru/RuO2 nanosheets for boosting hydrogen electrocatalysis
Juntao Zhang;Guomian Ren;Deyu Li;Qingyu Kong;Zhiwei Hu;Yong Xu;Suling Wang;Lu Wang;Maofeng Cao;Xiaoqing Huang-State Key Laboratory of Physical Chemistry of Solid Surfaces,College of Chemistry and Chemical Engineering,Xiamen University,Xiamen 361005,China;Guangzhou Key Laboratory of Low-Dimensional Materials and Energy Storage Devices,Collaborative Innovation Center of Advanced Energy Materials,School of Materials and Energy,Guangdong University of Technology,Guangzhou 510006,China;Institute of Functional Nano&Soft Materials,Jiangsu Key Laboratory for Carbon-Based Functional Materials&Devices,Soochow University,Suzhou 215123,China;Société Civile Synchrotron SOLEIL,L'Orme des Merisiers,Saint-Aubin 91192,France;School of Physics Science and Information Engineering,Shandong Key Laboratory of Optical Communication Science and Technology,Liaocheng University,Liaocheng 252059,China;Max Planck Institute for Chemical Physics of Solids,Dresden 01187,Germany
Electrochemical hydrogen-storage capacity of graphene can achieve a carbon-hydrogen atomic ratio of 1∶1
Quanfeng He;Lanping Zeng;Lianhuan Han;Juan Peng;Matthew M.Sartin;Yuan-Zhi Tan;Dongping Zhan;Zhong-Qun Tian-State Key Laboratory of Physical Chemistry of Solid Surfaces;Fujian Science & Technology Innovation Laboratory for Energy Materials of China;Engineering Research Center of Electrochemical Technologies of Ministry of Education;Graphene Industry and Engineering Research Institute;Department of Chemistry, College of Chemistry and Chemical Engineering;Department of Mechanical and Electrical Engineering, School of Aerospace Engineering, Xiamen University, Xiamen 361005, China;Department of Chemistry, College of Chemistry and Chemical Engineering, Ningxia University, Yinchuan 750021, China
机标中图分类号,由域田数据科技根据网络公开资料自动分析生成,仅供学习研究参考。