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典型文献
Ultrafast imaging of terahertz electric waveforms using quantum dots
文献摘要:
Microscopic electric fields govern the majority of elementary excitations in condensed matter and drive electronics at frequencies approaching the Terahertz (THz) regime.However,only few imaging schemes are able to resolve sub-wavelength fields in the THz range,such as scanning-probe techniques,electro-optic sampling,and ultrafast electron microscopy.Still,intrinsic constraints on sample geometry,acquisition speed and field strength limit their applicability.Here,we harness the quantum-confined Stark-effect to encode ultrafast electric near-fields into colloidal quantum dot luminescence.Our approach,termed Quantum-probe Field Microscopy (QFIM),combines far-field imaging of visible photons with phase-resolved sampling of electric waveforms.By capturing ultrafast movies,we spatio-temporally resolve a Terahertz resonance inside a bowtie antenna and unveil the propagation of a Terahertz waveguide excitation deeply in the sub-wavelength regime.The demonstrated QFIM approach is compatible with strong-field excitation and sub-micrometer resolution—introducing a direct route towards ultrafast field imaging of complex nanodevices in-operando.
文献关键词:
作者姓名:
Moritz B.Heindl;Nicholas Kirkwood;Tobias Lauster;Julia A.Lang;Markus Retsch;Paul Mulvaney;Georg Herink
作者机构:
Experimental Physics Ⅷ-Ultrafast Dynamics,University of Bayreuth,Bayreuth,Germany;ARC Centre of Excellence in Exciton Science,School of Chemistry,University of Melbourne,Melbourne,Australia;Physical Chemistry Ⅰ,University of Bayreuth,Bayreuth,Germany
引用格式:
[1]Moritz B.Heindl;Nicholas Kirkwood;Tobias Lauster;Julia A.Lang;Markus Retsch;Paul Mulvaney;Georg Herink-.Ultrafast imaging of terahertz electric waveforms using quantum dots)[J].光:科学与应用(英文版),2022(01):63-68
A类:
QFIM
B类:
Ultrafast,imaging,terahertz,electric,waveforms,using,quantum,dots,Microscopic,fields,govern,majority,elementary,excitations,condensed,matter,drive,electronics,frequencies,approaching,Terahertz,THz,regime,However,only,few,schemes,are,able,sub,wavelength,range,such,scanning,probe,techniques,optic,sampling,ultrafast,microscopy,Still,intrinsic,constraints,sample,geometry,acquisition,speed,strength,limit,their,applicability,Here,harness,confined,Stark,effect,encode,near,into,colloidal,luminescence,Our,termed,Quantum,Field,Microscopy,combines,far,visible,photons,phase,resolved,By,capturing,movies,spatio,temporally,resonance,inside,bowtie,antenna,unveil,propagation,waveguide,deeply,demonstrated,compatible,strong,micrometer,resolution,introducing,direct,route,towards,complex,nanodevices,operando
AB值:
0.65578
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