首站-论文投稿智能助手
首页
期刊导航
职称导航
中图分类号
典型文献
Synergetic degradation of Methylene Blue through photocatalysis and Fenton reaction on two-dimensional molybdenite-Fe
文献摘要：
The greatest problem in conventional Fenton reaction is the slow production of ROS (reactive oxygen species) because of the inefficient Fe3+/Fe2+ conversion.Based on the extraordinary photo-response property of two-dimensional molybdenite (2DM),photogenerated electrons can be easy separated to accelerate the regeneration of Fe2+.In this work,Fe2+-anchored 2DM (2DM-Fe) was prepared and used as a heterogeneous Fenton catalyst to investigate the degradation efficiency to Methylene Blue (MB) in the presence of light.According to experi-mental results,2DM-Fe exhibited extraordinary catalytic activity in MB elimination,which ascribed to the synergetic effect of photogenerated carriers and anchored Fe2+ to H2O2 acti-vation.In addition,2DM-Fe showed nearly 100％ degradation efficiency to MB within 5 cycles with slight leaching amount of Mo and Fe ions,implying the strong stability and reusabil-ity in H2O2 system.Furthermore,the influences of H2O2 and 2DM-Fe dosages,pH values as well as the degradation efficiency to different dyes were also investigated.According to quenching experiments and EPR (electron paramagnetic resonance) test,the degradation mechanism of MB mainly ascribed to the oxidation of HO· and ·O2-.This finding provides a novel strategy to design rational Fenton catalyst and has great significance to water reme-diation in the future.
文献关键词：
中图分类号：
[1] 医药、卫生（R） / 药学（R9） / 药理学（R96） / 实验药理学（R965）
[2] 医药、卫生（R） / 基础医学（R3） / 病理学（R36） / 病理过程（R364）
[3] 数理科学和化学（O） / 力学（O3） / 振动理论（O32） / 非线性振动（O322）
作者姓名：
Chang Liu;Bingqiao Yang;Jianxin Chen;Feifei Jia;Shaoxian Song
作者机构：
Hubei Key Laboratory of Mineral Resources Processing and Environment,Wuhan University of Technology,Wuhan 430070,China;Xingfa School of Mining Engineering,Wuhan Institute of Technology,Wuhan 430073,China;School of Resources and Environmental Engineering,Wuhan University of Technology,Wuhan 430070,China
文献出处：
环境科学学报（英文版）
引用格式：
[1]Chang Liu;Bingqiao Yang;Jianxin Chen;Feifei Jia;Shaoxian Song-.Synergetic degradation of Methylene Blue through photocatalysis and Fenton reaction on two-dimensional molybdenite-Fe)[J].环境科学学报（英文版）,2022(01):11-23
A类：
2DM,reusabil,reme
B类：
Synergetic,degradation,Methylene,Blue,through,photocatalysis,Fenton,reaction,two,dimensional,molybdenite,greatest,problem,conventional,slow,production,ROS,reactive,oxygen,species,because,inefficient,Fe3+,Fe2+,conversion,Based,extraordinary,response,property,photogenerated,electrons,easy,separated,accelerate,regeneration,In,this,work,anchored,was,prepared,used,heterogeneous,catalyst,efficiency,MB,presence,According,mental,results,exhibited,catalytic,activity,elimination,which,ascribed,synergetic,effect,carriers,H2O2,vation,addition,showed,nearly,within,cycles,slight,leaching,amount,Mo,ions,implying,strong,stability,system,Furthermore,influences,dosages,values,well,different,dyes,were,also,investigated,quenching,experiments,EPR,paramagnetic,resonance,mechanism,mainly,oxidation,HO,This,finding,provides,novel,strategy,design,rational,has,significance,water,diation,future
AB值：
0.546833
相似文献
In-situ synthesis of N,S co-doped hollow carbon microspheres for efficient catalytic oxidation of organic contaminants
Yongbing Xie;Ya Liu;Yujie Yao;Yanchun Shi;Binran Zhao;Yuxian Wang-State Key Laboratory of Vanadium and Titanium Resources Comprehensive Utilization,Panzhihua 617000,China;CAS Key Laboratory of Green Process&Engineering,Beijing Engineering Research Center of Process Pollution Control,Institute of Process Engineering,Chinese Academy of Sciences,Beijing 100190,China;State Key Laboratory of Heavy Oil Processing,State Key Laboratory of Petroleum Pollution Control,China University of Petroleum-Beijing,Beijing 102249,China;School of Chemical Engineering and Advanced Materials,The University of Adelaide,Adelaide,SA 5005,Australia;School of Chemical Engineering,Northwest University,Xi'an 710069,China
Molybdenum phosphide(MoP)with dual active sites for the degradation of diclofenac in Fenton-like system
Xiuying Li;Shuangqiu Huang;Huaihao Xu;Yuepeng Deng;Zhu Wang;Zhao-Qing Liu-Key Laboratory for Water Quality and Conservation of the Pearl River Delta,Ministry of Education,Guangzhou Key Laboratory for Clean Energy and Materials,Institute of Environmental Research at Greater Bay,Guangzhou University,Guangzhou 510006,China;State Key Laboratory of Pollution Control and Resource Reuse,School of the Environment,Nanjing University,Nanjing 210023,China;School of Chemistry and Chemical Engineering,Institute of Clean Energy and Materials,Guangzhou Key Laboratory for Clean Energy and Materials,Key Laboratory for Water Quality and Conservation of the Pearl River Delta,Ministry of Education,Guangzhou University,Guangzhou 510006,China
Rationally designed Ta3N5/BiOCl S-scheme heterojunction with oxygen vacancies for elimination of tetracycline antibiotic and Cr(Ⅵ):Performance,toxicity evaluation and mechanism insight
Shijie Li;Mingjie Cai;Chunchun Wang;Yanping Liu;Neng Li;Peng Zhang;Xin Li-Key Laboratory of Health Risk Factors for Seafood of Zhejiang Province,National Engineering Research Center for Marine Aquaculture,College of Marine Science and Technology,Zhejiang Ocean University,Zhoushan 316022,China;Institute of Innovation&Application,Zhejiang Ocean University,Zhoushan 316022,China;State Key Laboratory of Silicate Materials for Architectures,Wuhan University of Technology,Wuhan 430070,China;State Center for International Cooperation on Designer Low-Carbon&Environmental Materials(CDLCEM),School of Materials Science and Engineering,Zhengzhou University,Zhengzhou 450001,China;Institute of Biomass Engineering,Key Laboratory of Energy Plants Resource and Utilization,Ministry of Agriculture and Rural Affairs,South China Agricultural University,Guangzhou 510642,China
机标中图分类号，由域田数据科技根据网络公开资料自动分析生成，仅供学习研究参考。
客服邮箱：957655803@qq.com
渝公网安备：50011902000454号
ICP备案号：渝ICP备2023002303号
重庆域田数据科技有限公司©版权所有
官方客服